Outside Back Cover: The Importance of Si─ONa─Al Moieties in Fe/ZSM-5 Zeolite Catalysts for Selective Oxidation of Methane to Acetic Acid (Angew. Chem. 40/2025)
Xinyu Zhao, Haibin Yin, Hongfei Lin, Zijin Dai, Xin Chen, Wenlong Wu, Hongliang Li, Bo Wu, Jie Zeng
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引用次数: 0
Abstract
The image highlights electron transfer from Si─ONa─Al moieties to iron active sites in the Fe/ZSM-5-0.25Na driving selective C─C coupling between methane and CO, efficiently steering the reaction toward acetic acid formation. In their Research Article (e202511056), Jie Zeng, Bo Wu et al. demonstrate a strategy to bypass traditional Brønsted acid dependency, employing metal-electronic modulation to enhance catalytic efficiency, and to establishes an innovative pathway for methane conversion.
该图像突出了Fe/ZSM-5-0.25Na中Si─ONa─Al基团向铁活性位点的电子转移，驱动甲烷和CO之间的选择性C─C偶联，有效地引导反应形成乙酸。在他们的研究文章（e202511056）中，Jie Zeng， Bo Wu等人展示了一种绕过传统Brønsted酸依赖的策略，采用金属电子调制来提高催化效率，并建立了一种创新的甲烷转化途径。
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