The Nature of Hygroscopicity of Aerosol Haze Particles over Beijing

IF 0.9 Q4 OPTICS
G. B. Pronchev, A. N. Yermakov
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引用次数: 0

Abstract

Atmospheric aerosols have a significant impact on air quality, climate, and human health. The comparison of gaseous impurity and ionic composition monitoring data in the surface atmosphere over Antwerp and Beijing showed that the hygroscopicity level of dense haze particles over Beijing in winter is determined by the depth of heterogeneous reactions of sulfate and nitrate formation. The paper discusses the dynamics and mechanisms of these nonphotochemical processes, as well as the features of their coupling in a haze-polluted atmosphere. Their rapid occurrence in particles in combination with the uptake of water vapor from the air causes abnormally high mass concentrations of aerosol and their variability during the haze period over Beijing. The results are necessary for forecasting the occurrence of dense hazes, as well as for constructing models of transport of gas and aerosol microimpurities in the atmosphere.

Abstract Image

北京地区雾霾颗粒的吸湿性
大气气溶胶对空气质量、气候和人类健康有重大影响。通过对安特卫普和北京地面大气中气体杂质和离子组成监测数据的比较,发现北京冬季雾霾的吸湿程度是由硫酸盐和硝酸盐形成的非均相反应的深度决定的。本文讨论了这些非光化学过程的动力学和机理,以及它们在雾霾污染大气中的耦合特征。它们在颗粒中迅速出现,再加上空气中水蒸气的吸收,导致了北京雾霾期间气溶胶质量浓度异常高及其变化。这些结果对于预测密集雾霾的发生,以及建立大气中气体和气溶胶微杂质的输送模型是必要的。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
CiteScore
2.40
自引率
42.90%
发文量
84
期刊介绍: Atmospheric and Oceanic Optics  is an international peer reviewed journal that presents experimental and theoretical articles relevant to a wide range of problems of atmospheric and oceanic optics, ecology, and climate. The journal coverage includes: scattering and transfer of optical waves, spectroscopy of atmospheric gases, turbulent and nonlinear optical phenomena, adaptive optics, remote (ground-based, airborne, and spaceborne) sensing of the atmosphere and the surface, methods for solving of inverse problems, new equipment for optical investigations, development of computer programs and databases for optical studies. Thematic issues are devoted to the studies of atmospheric ozone, adaptive, nonlinear, and coherent optics, regional climate and environmental monitoring, and other subjects.
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