{"title":"A distribution-free interval estimation method for lithium-ion battery state of health","authors":"Xiaoqiong Pang, Ziyao Guo, Jianfang Jia, Jie Wen, Xiaojie Li, Jianchao Zeng, Jiashuo Zhang","doi":"10.1007/s11581-025-06470-3","DOIUrl":null,"url":null,"abstract":"<div><p>In order to estimate the state of health (SOH) of lithium-ion batteries, traditional methods are often based on distributional assumptions that may not match the actual situation and lead to the construction of prediction intervals (PIs) that are unreliable. To this end, a distribution-free interval estimation strategy for SOH in lithium-ion batteries is proposed in this paper, which aims to efficiently construct high-quality PIs. To ensure compatibility with the gradient descent (GD) algorithm and to overcome the previous reliance on meta-heuristics, the loss function is redesigned and the PI centre is innovatively incorporated into the optimization objective. The aim is to obtain high-quality PIs for a more comprehensive assessment of their quality. Through the validation of the NASA dataset and the CALCE dataset, the results show that the proposed method improves the comprehensive evaluation metric <i>P</i> by an average of 40.69% compared to the traditional lower upper bound estimation (LUBE) method and improves the mean PI centre deviation (MPICD) metric by 13.60% compared to the model that does not consider the PI centre.</p></div>","PeriodicalId":599,"journal":{"name":"Ionics","volume":"31 8","pages":"7939 - 7952"},"PeriodicalIF":2.6000,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Ionics","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s11581-025-06470-3","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
In order to estimate the state of health (SOH) of lithium-ion batteries, traditional methods are often based on distributional assumptions that may not match the actual situation and lead to the construction of prediction intervals (PIs) that are unreliable. To this end, a distribution-free interval estimation strategy for SOH in lithium-ion batteries is proposed in this paper, which aims to efficiently construct high-quality PIs. To ensure compatibility with the gradient descent (GD) algorithm and to overcome the previous reliance on meta-heuristics, the loss function is redesigned and the PI centre is innovatively incorporated into the optimization objective. The aim is to obtain high-quality PIs for a more comprehensive assessment of their quality. Through the validation of the NASA dataset and the CALCE dataset, the results show that the proposed method improves the comprehensive evaluation metric P by an average of 40.69% compared to the traditional lower upper bound estimation (LUBE) method and improves the mean PI centre deviation (MPICD) metric by 13.60% compared to the model that does not consider the PI centre.
期刊介绍:
Ionics is publishing original results in the fields of science and technology of ionic motion. This includes theoretical, experimental and practical work on electrolytes, electrode, ionic/electronic interfaces, ionic transport aspects of corrosion, galvanic cells, e.g. for thermodynamic and kinetic studies, batteries, fuel cells, sensors and electrochromics. Fast solid ionic conductors are presently providing new opportunities in view of several advantages, in addition to conventional liquid electrolytes.