Design Strategies and Performance Enhancement Techniques for LiFePO4-Based Li Metal Battery Systems

IF 3.2 4区 工程技术 Q2 CHEMISTRY, MULTIDISCIPLINARY
Jiwon Choi, Jihyeon Kang, Chaerim Kim, Chaerin Jung, Raehyeong Lee, Mihee Park, Minjoon Park
{"title":"Design Strategies and Performance Enhancement Techniques for LiFePO4-Based Li Metal Battery Systems","authors":"Jiwon Choi,&nbsp;Jihyeon Kang,&nbsp;Chaerim Kim,&nbsp;Chaerin Jung,&nbsp;Raehyeong Lee,&nbsp;Mihee Park,&nbsp;Minjoon Park","doi":"10.1007/s11814-025-00446-9","DOIUrl":null,"url":null,"abstract":"<div><p>LiFePO<sub>4</sub> (LFP) batteries are a promising choice for electric vehicles and energy storage systems owing to their excellent long cycle life, thermal stability, and high energy density. Various strategies have been studied, including advancements in LFP active materials, electrolyte additives, current collectors, and binders. Despite the ongoing research, the practical fabrication of both LFP cathodes and lithium metal anodes (LMAs) remains challenging, limiting their industrial application. In addition to advancements in cathode materials, extensive research has been dedicated to lithium (Li) metal batteries to improve energy density. However, challenges associated with Li metal anodes, such as Li volume expansion and dendrite growth, often result in short circuits during Li plating/stripping processes. To address these issues, various strategies have been explored, including enhancing the lithiophilicity of Cu current collectors and utilizing 3D host structures. This review discusses the design and strategies for performance enhancement of various LFP electrodes and Li metal and, with emphasis on the development of materials and cell design.</p></div>","PeriodicalId":684,"journal":{"name":"Korean Journal of Chemical Engineering","volume":"42 7","pages":"1427 - 1451"},"PeriodicalIF":3.2000,"publicationDate":"2025-04-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Korean Journal of Chemical Engineering","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s11814-025-00446-9","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

LiFePO4 (LFP) batteries are a promising choice for electric vehicles and energy storage systems owing to their excellent long cycle life, thermal stability, and high energy density. Various strategies have been studied, including advancements in LFP active materials, electrolyte additives, current collectors, and binders. Despite the ongoing research, the practical fabrication of both LFP cathodes and lithium metal anodes (LMAs) remains challenging, limiting their industrial application. In addition to advancements in cathode materials, extensive research has been dedicated to lithium (Li) metal batteries to improve energy density. However, challenges associated with Li metal anodes, such as Li volume expansion and dendrite growth, often result in short circuits during Li plating/stripping processes. To address these issues, various strategies have been explored, including enhancing the lithiophilicity of Cu current collectors and utilizing 3D host structures. This review discusses the design and strategies for performance enhancement of various LFP electrodes and Li metal and, with emphasis on the development of materials and cell design.

lifepo4基锂金属电池系统的设计策略与性能提升技术
LiFePO4 (LFP)电池具有优良的长循环寿命、热稳定性和高能量密度,是电动汽车和储能系统的理想选择。研究了各种策略,包括LFP活性材料、电解质添加剂、集流器和粘合剂的进展。尽管研究正在进行中,但LFP阴极和锂金属阳极(lma)的实际制造仍然具有挑战性,限制了它们的工业应用。除了阴极材料的进步,锂(Li)金属电池也得到了广泛的研究,以提高能量密度。然而,与锂金属阳极相关的挑战,如锂体积膨胀和枝晶生长,经常导致在锂电镀/剥离过程中短路。为了解决这些问题,研究人员探索了各种策略,包括增强Cu集热器的亲石性和利用3D宿主结构。本文讨论了各种LFP电极和锂金属的设计和性能增强策略,重点介绍了材料和电池设计的发展。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Korean Journal of Chemical Engineering
Korean Journal of Chemical Engineering 工程技术-工程:化工
CiteScore
4.60
自引率
11.10%
发文量
310
审稿时长
4.7 months
期刊介绍: The Korean Journal of Chemical Engineering provides a global forum for the dissemination of research in chemical engineering. The Journal publishes significant research results obtained in the Asia-Pacific region, and simultaneously introduces recent technical progress made in other areas of the world to this region. Submitted research papers must be of potential industrial significance and specifically concerned with chemical engineering. The editors will give preference to papers having a clearly stated practical scope and applicability in the areas of chemical engineering, and to those where new theoretical concepts are supported by new experimental details. The Journal also regularly publishes featured reviews on emerging and industrially important subjects of chemical engineering as well as selected papers presented at international conferences on the subjects.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信