Impact of clean fracturing fluids on sustainable coalbed methane mining

IF 7.8 2区 环境科学与生态学 Q1 ENGINEERING, CHEMICAL
Qian Zhang , Feng Cai , Yaxin Liu , Xinjian Dang , Yandong Wang , Yong Luo
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Abstract

Modification of coal seams using fracturing fluids is a critical means to enhance methane extraction efficiency from low-permeability coal reservoirs in China. Nevertheless, some of the existing fracturing fluids pose risks of groundwater contamination due to their toxicity and corrosiveness, which severely limits the engineering application of this technology. Three types of green and clean fracturing fluids were developed in this paper using Huainan bituminous coal in China as the research object. Through the combination of macroscopic experiment and molecular dynamics simulation, the systematic study of the changing law of molecular structure, which has an important implication on the gas desorption and permeability characteristics of the treated coal samples, was carried out, and the fracturing fluids suitable for the test coal seam with high efficiency, environmental protection and safety were preferred. The clean fracturing fluid effectively regulates the microcrystalline structure of coal, reduces methane adsorption energy, and improves gas migration pathways. Simultaneously, it enhances electrostatic interactions and interfacial electron transfer to decrease methane-coal interaction energy, thereby synergistically improving methane migration efficiency. The findings are vital for promoting clean production, efficient extraction and safe production of coalbed methane.
清洁压裂液对煤层气可持续开采的影响
利用压裂液对煤层进行改造是提高中国低渗透煤储层甲烷开采效率的重要手段。然而,现有的一些压裂液由于其毒性和腐蚀性而存在污染地下水的风险,这严重限制了该技术的工程应用。以淮南烟煤为研究对象,开发了三种绿色清洁压裂液。通过宏观实验与分子动力学模拟相结合的方法,系统研究了分子结构的变化规律,对处理后煤样的气体解吸渗透特性具有重要意义,优选出高效、环保、安全、适合试验煤层的压裂液。清洁压裂液有效调节了煤的微晶结构,降低了甲烷吸附能,改善了天然气运移途径。同时,增强静电相互作用和界面电子传递,降低甲烷-煤相互作用能,协同提高甲烷迁移效率。这一发现对于促进煤层气的清洁生产、高效开采和安全生产具有重要意义。
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来源期刊
Process Safety and Environmental Protection
Process Safety and Environmental Protection 环境科学-工程:化工
CiteScore
11.40
自引率
15.40%
发文量
929
审稿时长
8.0 months
期刊介绍: The Process Safety and Environmental Protection (PSEP) journal is a leading international publication that focuses on the publication of high-quality, original research papers in the field of engineering, specifically those related to the safety of industrial processes and environmental protection. The journal encourages submissions that present new developments in safety and environmental aspects, particularly those that show how research findings can be applied in process engineering design and practice. PSEP is particularly interested in research that brings fresh perspectives to established engineering principles, identifies unsolved problems, or suggests directions for future research. The journal also values contributions that push the boundaries of traditional engineering and welcomes multidisciplinary papers. PSEP's articles are abstracted and indexed by a range of databases and services, which helps to ensure that the journal's research is accessible and recognized in the academic and professional communities. These databases include ANTE, Chemical Abstracts, Chemical Hazards in Industry, Current Contents, Elsevier Engineering Information database, Pascal Francis, Web of Science, Scopus, Engineering Information Database EnCompass LIT (Elsevier), and INSPEC. This wide coverage facilitates the dissemination of the journal's content to a global audience interested in process safety and environmental engineering.
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