High Transmission Efficiency Hybrid Metal-Dielectric Metasurfaces for Mid-Infrared Spectroscopy.

IF 4.3 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Nanomaterials Pub Date : 2025-09-22 DOI:10.3390/nano15181456
Amr Soliman, Calum Williams, Timothy D Wilkinson
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引用次数: 0

Abstract

Mid-infrared (MIR) spectroscopy enables non-invasive identification of chemical species by probing absorption spectra associated with molecular vibrational modes, where spectral filters play a central role. Conventional plasmonic metasurfaces have been explored for MIR filtering in reflection and transmission modes but typically suffer from broad spectral profiles and low efficiencies. All-dielectric metasurfaces, although characterized by low intrinsic losses, are largely limited to reflection mode operation. To overcome these limitations, we propose a hybrid metal-dielectric metasurface that combines the advantages of both platforms while simplifying fabrication compared to conventional Fabry-Pérot filters. The proposed filter consists of silicon (Si) crosses atop gold (Au) square patches and demonstrates a transmission efficiency of 87% at the operating wavelength of 4.28 µm, with a full width half maximum (FWHM) as narrow as 43 nm and a quality factor of approximately 99.5 at λ = 4.28 μm. Numerical simulations attribute this performance to hybridization of Mie lattice resonances in both the gold patches and silicon crosses. By providing narrowband, high-transmission filtering in the MIR, the hybrid metasurface offers a compact and versatile platform for selective gas detection and imaging. This work establishes hybrid metal-dielectric metasurfaces as a promising direction for next-generation MIR spectroscopy.

用于中红外光谱的高透射效率混合金属-介电超表面。
中红外(MIR)光谱学通过探测与分子振动模式相关的吸收光谱来实现化学物种的非侵入性鉴定,其中光谱滤波器起着核心作用。传统的等离子体超表面已经在反射和透射模式下进行了MIR滤波,但通常存在光谱分布宽和效率低的问题。全介电超表面虽然具有低本征损耗的特点,但主要局限于反射模式的工作。为了克服这些限制,我们提出了一种混合金属-介电超表面,它结合了两种平台的优点,同时与传统的法布里-普氏滤波器相比简化了制造。该滤波器由金(Au)方形贴片上的硅(Si)交叉组成,在4.28 μm工作波长下的传输效率为87%,全宽半最大(FWHM)窄至43 nm, λ = 4.28 μm处的质量因子约为99.5。数值模拟将这种性能归因于金片和硅交叉中的Mie晶格共振的杂化。通过在MIR中提供窄带,高传输滤波,混合超表面为选择性气体检测和成像提供了一个紧凑而通用的平台。这项工作建立了混合金属-介电超表面作为下一代MIR光谱的一个有前途的方向。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Nanomaterials
Nanomaterials NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
8.50
自引率
9.40%
发文量
3841
审稿时长
14.22 days
期刊介绍: Nanomaterials (ISSN 2076-4991) is an international and interdisciplinary scholarly open access journal. It publishes reviews, regular research papers, communications, and short notes that are relevant to any field of study that involves nanomaterials, with respect to their science and application. Thus, theoretical and experimental articles will be accepted, along with articles that deal with the synthesis and use of nanomaterials. Articles that synthesize information from multiple fields, and which place discoveries within a broader context, will be preferred. There is no restriction on the length of the papers. Our aim is to encourage scientists to publish their experimental and theoretical research in as much detail as possible. Full experimental or methodical details, or both, must be provided for research articles. Computed data or files regarding the full details of the experimental procedure, if unable to be published in a normal way, can be deposited as supplementary material. Nanomaterials is dedicated to a high scientific standard. All manuscripts undergo a rigorous reviewing process and decisions are based on the recommendations of independent reviewers.
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