Experimental Investigation of Borehole Sealing Efficiency in Coalbed Methane Extraction Using Controllable Slow-Release Materials

IF 3.9 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Yunfei Zuo, Bo Tan, Zixuan Jia, Hao Lu, Feng Du, Chunjing Han, Yu Wang, Qi Tang
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Abstract

The inadequate sealing of extraction boreholes significantly reduces gas extraction efficiency and hinders the effective prevention of gas disasters. This study presents a novel sealing material with adjustable slow-release properties. The seepage and sealing performances of materials with different mix ratios were tested to determine the optimal formulation. The underlying mechanism was further analyzed based on the materials’ physicochemical characteristics, and field experiments were conducted to validate the leakage control effectiveness of the controllable slow-release sealing material, thereby elucidating its mechanism for enhancing borehole sealing performance. The results indicate that the controllable slow-release sealing material with a water-to-material ratio of 4:1 performs best. The material consists primarily of montmorillonite, which is rich in SiO2 and Al2O3, and exhibits excellent permeability and sealing characteristics. The nano-oxides, in cooperation with the surfactant, impart the slow-release blocking properties to the material. Initially, the material exhibits low viscosity, with excellent fluidity and permeability, allowing it to infiltrate the microfractures of the coal seam. As the injection time increases, the cross-linking agent within the material progressively reacts to form a polymer gel with a defined strength. In addition, the material can obstruct newly formed fissures during the continued expansion of coal body fractures, thereby demonstrating an effective dynamic blocking performance. These findings provide reliable technological support for the continuous sealing of coal seam fractures and efficient gas extraction.

Abstract Image

可控缓释材料煤层气抽采封孔效率实验研究
抽采钻孔密封不良严重降低了瓦斯抽采效率,阻碍了瓦斯灾害的有效防治。本研究提出了一种具有可调缓释性能的新型密封材料。通过对不同配合比材料的渗流和密封性能进行试验,确定了最佳配合比配方。根据材料的物理化学特性,进一步分析其作用机理,并进行现场试验,验证可控缓释密封材料的防漏效果,阐明其提高井眼密封性能的机理。结果表明,水料比为4:1的可控缓释密封材料性能最好。该材料主要由富含SiO2和Al2O3的蒙脱土组成,具有良好的渗透性和密封性。纳米氧化物与表面活性剂合作,赋予材料缓释阻塞特性。物料初始粘度低,流动性和渗透性好,可以渗透到煤层微裂隙中。随着注射时间的增加,材料内的交联剂逐渐反应形成具有确定强度的聚合物凝胶。此外,在煤体裂隙持续扩展过程中,该材料还能封堵新形成的裂隙,具有有效的动态封堵性能。这些研究成果为煤层裂隙的连续密封和高效瓦斯开采提供了可靠的技术支撑。
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来源期刊
Langmuir
Langmuir 化学-材料科学:综合
CiteScore
6.50
自引率
10.30%
发文量
1464
审稿时长
2.1 months
期刊介绍: Langmuir is an interdisciplinary journal publishing articles in the following subject categories: Colloids: surfactants and self-assembly, dispersions, emulsions, foams Interfaces: adsorption, reactions, films, forces Biological Interfaces: biocolloids, biomolecular and biomimetic materials Materials: nano- and mesostructured materials, polymers, gels, liquid crystals Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do? Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*. This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).
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