Asymmetric Contact van der Waals Ferroelectric Transistors for Self-Powered Multifunctional Artificial Visual System

IF 16 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
ACS Nano Pub Date : 2025-09-25 DOI:10.1021/acsnano.5c12376
Rajiv Kumar Pandey, , , Sungpyo Baek, , , Nayeong Lee, , , Sang-Min Lee, , and , Sungjoo Lee*, 
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Abstract

The development of self-powered artificial visual systems capable of emulating the multifunctionality of the human eye, such as light adaptation, optical memory, and in-sensor computing, is pivotal for next-generation intelligent bionic technologies. In this study, we present a van der Waals ferroelectric field-effect transistor (vdW-FeFET) based on an asymmetric contact α-In2Se3/h-BN/CIPS heterostructure, which operates entirely in a self-powered mode. By harnessing the intrinsic opto-ferroelectric coupling of α-In2Se3 and the built-in electric fields induced by asymmetric source–drain contact areas, the device exhibits a range of neuromorphic visual behaviors, including visible light sensing and adaptation (405–660 nm), wavelength-dependent color differentiation, and robust optical memory capabilities. The combined effects of photopyroelectric and photothermoelectric mechanisms enable dynamic modulation of the photocurrent, facilitating visual adaptations analogous to biological systems. The device further demonstrates pronounced synaptic characteristics, such as a high paired-pulse facilitation index (∼180%) and memory consolidation from short- to long-term states under repetitive optical stimulation. In particular, pattern recognition is achieved without any external bias, showcasing the potential for autonomous visual signal processing. This work presents a multifunctional, energy-efficient platform for bioinspired vision systems, offering a promising pathway toward neuromorphic computing and next-generation optoelectronic intelligence.

Abstract Image

Abstract Image

用于自供电多功能人工视觉系统的非对称接触范德华铁电晶体管
开发能够模拟人眼多功能的自供电人工视觉系统,如光适应、光存储器和传感器内计算,是下一代智能仿生技术的关键。在这项研究中,我们提出了一种基于非对称接触α-In2Se3/h-BN/CIPS异质结构的范德华铁电场效应晶体管(vdW-FeFET),该晶体管完全在自供电模式下工作。通过利用α-In2Se3的固有光-铁电耦合和不对称源-泄接触区引起的内置电场,该器件表现出一系列神经形态的视觉行为,包括可见光感知和适应(405-660 nm)、波长相关的颜色区分和强大的光存储能力。光热光电和光热电机制的联合作用使光电流能够动态调制,促进类似于生物系统的视觉适应。该装置进一步展示了明显的突触特性,例如高配对脉冲促进指数(~ 180%)和记忆在重复光刺激下从短期到长期状态的巩固。特别是,模式识别是在没有任何外部偏差的情况下实现的,展示了自主视觉信号处理的潜力。这项工作为生物视觉系统提供了一个多功能、节能的平台,为神经形态计算和下一代光电智能提供了一条有前途的途径。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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