{"title":"Asymmetric Contact van der Waals Ferroelectric Transistors for Self-Powered Multifunctional Artificial Visual System","authors":"Rajiv Kumar Pandey, , , Sungpyo Baek, , , Nayeong Lee, , , Sang-Min Lee, , and , Sungjoo Lee*, ","doi":"10.1021/acsnano.5c12376","DOIUrl":null,"url":null,"abstract":"<p >The development of self-powered artificial visual systems capable of emulating the multifunctionality of the human eye, such as light adaptation, optical memory, and in-sensor computing, is pivotal for next-generation intelligent bionic technologies. In this study, we present a van der Waals ferroelectric field-effect transistor (vdW-FeFET) based on an asymmetric contact α-In<sub>2</sub>Se<sub>3</sub>/h-BN/CIPS heterostructure, which operates entirely in a self-powered mode. By harnessing the intrinsic opto-ferroelectric coupling of α-In<sub>2</sub>Se<sub>3</sub> and the built-in electric fields induced by asymmetric source–drain contact areas, the device exhibits a range of neuromorphic visual behaviors, including visible light sensing and adaptation (405–660 nm), wavelength-dependent color differentiation, and robust optical memory capabilities. The combined effects of photopyroelectric and photothermoelectric mechanisms enable dynamic modulation of the photocurrent, facilitating visual adaptations analogous to biological systems. The device further demonstrates pronounced synaptic characteristics, such as a high paired-pulse facilitation index (∼180%) and memory consolidation from short- to long-term states under repetitive optical stimulation. In particular, pattern recognition is achieved without any external bias, showcasing the potential for autonomous visual signal processing. This work presents a multifunctional, energy-efficient platform for bioinspired vision systems, offering a promising pathway toward neuromorphic computing and next-generation optoelectronic intelligence.</p>","PeriodicalId":21,"journal":{"name":"ACS Nano","volume":"19 39","pages":"35071–35080"},"PeriodicalIF":16.0000,"publicationDate":"2025-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Nano","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsnano.5c12376","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The development of self-powered artificial visual systems capable of emulating the multifunctionality of the human eye, such as light adaptation, optical memory, and in-sensor computing, is pivotal for next-generation intelligent bionic technologies. In this study, we present a van der Waals ferroelectric field-effect transistor (vdW-FeFET) based on an asymmetric contact α-In2Se3/h-BN/CIPS heterostructure, which operates entirely in a self-powered mode. By harnessing the intrinsic opto-ferroelectric coupling of α-In2Se3 and the built-in electric fields induced by asymmetric source–drain contact areas, the device exhibits a range of neuromorphic visual behaviors, including visible light sensing and adaptation (405–660 nm), wavelength-dependent color differentiation, and robust optical memory capabilities. The combined effects of photopyroelectric and photothermoelectric mechanisms enable dynamic modulation of the photocurrent, facilitating visual adaptations analogous to biological systems. The device further demonstrates pronounced synaptic characteristics, such as a high paired-pulse facilitation index (∼180%) and memory consolidation from short- to long-term states under repetitive optical stimulation. In particular, pattern recognition is achieved without any external bias, showcasing the potential for autonomous visual signal processing. This work presents a multifunctional, energy-efficient platform for bioinspired vision systems, offering a promising pathway toward neuromorphic computing and next-generation optoelectronic intelligence.
期刊介绍:
ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.