{"title":"Online improving NOX concentration prediction at SCR system outlet through continual learning","authors":"Peng Chen , Baochang Xu , Wei He , Hongtao Hu","doi":"10.1016/j.jtice.2025.106417","DOIUrl":null,"url":null,"abstract":"<div><h3>Background</h3><div>Accurately predicting NO<sub>X</sub> concentration at SCR system outlet is crucial for optimizing process parameters and reducing NO<sub>X</sub> emissions. Existing prediction models often struggle to maintain accurate long-term online predictions when operating conditions change and new data arrive. Therefore, frequent model updates are required in practical applications. However, new models often exhibit catastrophic forgetting of learned patterns, leading to a deterioration in NO<sub>X</sub> concentration prediction accuracy.</div></div><div><h3>Methods</h3><div>A novel continual learning algorithm, termed TDIR, is proposed. This algorithm dynamically identifies historical temporal samples that are most susceptible to interference from new data and prioritizes their replay. The TDIR algorithm is integrated with the iTransformer architecture to establish TDIRformer, an online self-updating model for NO<sub>X</sub> emission prediction. The model utilizes variate tokens to capture cross-feature correlations, effectively addressing prediction inaccuracies caused by multivariate coupling. It also employs the TDIR algorithm for online updates, which mitigates catastrophic forgetting and improves the prediction accuracy of NO<sub>X</sub> concentrations.</div></div><div><h3>Significant findings</h3><div>Experimental results show that TDIRformer significantly outperforms LSTM, Informer, PatchTST, and iTransformer, while TDIR also surpasses the continual learning methods EWC and MAS. Additionally, the TDIR algorithm demonstrates strong generalization capability, achieving RMSE reductions of 10.7 %, 9.3 %, and 11.9 % when applied to LSTM, Informer, and PatchTST models, respectively.</div></div>","PeriodicalId":381,"journal":{"name":"Journal of the Taiwan Institute of Chemical Engineers","volume":"179 ","pages":"Article 106417"},"PeriodicalIF":6.3000,"publicationDate":"2025-09-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of the Taiwan Institute of Chemical Engineers","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1876107025004675","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Background
Accurately predicting NOX concentration at SCR system outlet is crucial for optimizing process parameters and reducing NOX emissions. Existing prediction models often struggle to maintain accurate long-term online predictions when operating conditions change and new data arrive. Therefore, frequent model updates are required in practical applications. However, new models often exhibit catastrophic forgetting of learned patterns, leading to a deterioration in NOX concentration prediction accuracy.
Methods
A novel continual learning algorithm, termed TDIR, is proposed. This algorithm dynamically identifies historical temporal samples that are most susceptible to interference from new data and prioritizes their replay. The TDIR algorithm is integrated with the iTransformer architecture to establish TDIRformer, an online self-updating model for NOX emission prediction. The model utilizes variate tokens to capture cross-feature correlations, effectively addressing prediction inaccuracies caused by multivariate coupling. It also employs the TDIR algorithm for online updates, which mitigates catastrophic forgetting and improves the prediction accuracy of NOX concentrations.
Significant findings
Experimental results show that TDIRformer significantly outperforms LSTM, Informer, PatchTST, and iTransformer, while TDIR also surpasses the continual learning methods EWC and MAS. Additionally, the TDIR algorithm demonstrates strong generalization capability, achieving RMSE reductions of 10.7 %, 9.3 %, and 11.9 % when applied to LSTM, Informer, and PatchTST models, respectively.
期刊介绍:
Journal of the Taiwan Institute of Chemical Engineers (formerly known as Journal of the Chinese Institute of Chemical Engineers) publishes original works, from fundamental principles to practical applications, in the broad field of chemical engineering with special focus on three aspects: Chemical and Biomolecular Science and Technology, Energy and Environmental Science and Technology, and Materials Science and Technology. Authors should choose for their manuscript an appropriate aspect section and a few related classifications when submitting to the journal online.