Visualization experiment and numerical analysis of supercritical CO2 flow inside porous chip: Effect of heat transfer and porous structures

IF 4.4 3区 工程技术 Q2 CHEMISTRY, PHYSICAL
Jiaxin Liu , Mengshuai Chen , Rachid Bennacer , Lin Chen
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Abstract

Carbon dioxide (CO2) geological sequestration is one of the key methods to reduce atmospheric carbon emissions, yet the migration mechanisms of CO₂ within reservoirs remain unclear. This study systematically investigates the flow and heat transfer characteristics of supercritical CO₂ (sCO₂) in porous media through integrated optical visualization experiments and numerical simulations. Experimental results show that under supercritical conditions (pressure: 8.2–8.6 MPa, temperature: 32–34 °C), increasing the outlet pressure enhances momentum exchange but reduces flow uniformity, whereas raising the inlet temperature reduces fluid viscosity and smoothens density gradients, thereby improving flow homogeneity. Numerical simulations further reveal that under supercritical conditions (8.5 MPa, 305.15–318.15 K), boundary parameters including the inlet Reynolds number, inlet temperature, and wall heat flux exhibit non-monotonic influence patterns on the heat transfer coefficient (HTC), with an optimal range identified for each parameter. Exceeding this range leads to a significant reduction in HTC by 75–94 %. Under transcritical conditions (7.5–9.0 MPa, 303.15 K), the structure of the porous media effectively suppresses disturbances caused by thermophysical nonlinearities of sCO₂ through flow inertia, enabling the local heat transfer coefficient to maintain strong robustness against variations in outlet pressure and heat flux.
多孔切屑内超临界CO2流动的可视化实验与数值分析:传热与多孔结构的影响
二氧化碳(CO2)地质封存是减少大气碳排放的关键方法之一,但CO2在水库中的迁移机制尚不清楚。通过综合光学可视化实验和数值模拟,系统研究了超临界CO₂(sCO₂)在多孔介质中的流动和换热特性。实验结果表明,在超临界工况下(压力8.2 ~ 8.6 MPa,温度32 ~ 34℃),增大出口压力可增强动量交换,但会降低流动均匀性,而提高进口温度可降低流体粘度,平滑密度梯度,从而改善流动均匀性。数值模拟进一步表明,在超临界条件下(8.5 MPa, 305.15-318.15 K),包括进口雷诺数、进口温度和壁面热流密度在内的边界参数对换热系数(HTC)表现出非单调的影响模式,并确定了每个参数的最优范围。超过这个范围会导致HTC显著减少75 - 94% %。在跨临界条件下(7.5-9.0 MPa, 303.15 K),多孔介质的结构通过流动惯性有效地抑制了sCO₂热物理非线性引起的扰动,使局部换热系数对出口压力和热流密度的变化保持较强的鲁棒性。
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来源期刊
Journal of Supercritical Fluids
Journal of Supercritical Fluids 工程技术-工程:化工
CiteScore
7.60
自引率
10.30%
发文量
236
审稿时长
56 days
期刊介绍: The Journal of Supercritical Fluids is an international journal devoted to the fundamental and applied aspects of supercritical fluids and processes. Its aim is to provide a focused platform for academic and industrial researchers to report their findings and to have ready access to the advances in this rapidly growing field. Its coverage is multidisciplinary and includes both basic and applied topics. Thermodynamics and phase equilibria, reaction kinetics and rate processes, thermal and transport properties, and all topics related to processing such as separations (extraction, fractionation, purification, chromatography) nucleation and impregnation are within the scope. Accounts of specific engineering applications such as those encountered in food, fuel, natural products, minerals, pharmaceuticals and polymer industries are included. Topics related to high pressure equipment design, analytical techniques, sensors, and process control methodologies are also within the scope of the journal.
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