Carbon capture, utilization, and storage for sustainable construction: Insights into CO2 mixing, curing, and mineralization

Kamran Aghaee
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Abstract

Given the substantial share of global CO2 emissions attributable to construction materials, especially cement, there is rising interest in harnessing CO2 to enhance cementitious composites and generate value‑added products. Strategic carbon capture, utilization, and storage (CCUS) techniques including CO2 mixing, curing, and mineralization can improve the macro‑mechanical performance and microstructure of cement‑based materials and enable the development of novel binders and construction materials. This article synthesizes current CCUS techniques applicable to construction materials, particularly concrete composites, and elaborates on key parameters affecting their effectiveness. The findings suggest that CO2 mineralization is more effective than CO2 mixing and curing, revealing its considerable potential for producing carbon-sink materials from construction and industrial by-products that support circularity through reuse and closing the loop in construction. However, this approach still faces challenges related to scale-up and economic feasibility. This study compares and identifies the optimal implementation conditions to maximize material performance and production efficiency, while also evaluating the economic and environmental impacts of the technologies, with a focus on advancing circularity in construction.

Abstract Image

可持续建筑的碳捕获、利用和储存:对二氧化碳混合、固化和矿化的见解
鉴于建筑材料(尤其是水泥)在全球二氧化碳排放中所占的很大份额,人们对利用二氧化碳来增强水泥复合材料和产生增值产品的兴趣日益浓厚。包括二氧化碳混合、固化和矿化在内的战略性碳捕获、利用和封存(CCUS)技术可以改善水泥基材料的宏观力学性能和微观结构,并使新型粘合剂和建筑材料的开发成为可能。本文综合了目前适用于建筑材料,特别是混凝土复合材料的CCUS技术,并详细阐述了影响其有效性的关键参数。研究结果表明,二氧化碳矿化比二氧化碳混合和固化更有效,揭示了它在从建筑和工业副产品中生产碳汇材料方面的巨大潜力,这些材料通过再利用和封闭建筑中的循环来支持循环。然而,这种方法仍然面临着规模扩大和经济可行性方面的挑战。本研究比较并确定了最佳实施条件,以最大限度地提高材料性能和生产效率,同时也评估了这些技术的经济和环境影响,重点是推进建筑中的循环。
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