Toward Reliable and Reproducible Research in Organic Photocatalysis by Carbon Nitride

IF 13.1 1区 化学 Q1 CHEMISTRY, PHYSICAL
Gaia Grando, , , Giuseppe Sportelli, , , Gaia Castellani, , , Giacomo Filippini, , , Maurizio Prato, , , Michele Melchionna*, , and , Paolo Fornasiero*, 
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Abstract

The rate of scientific publications has grown exponentially over the past few decades, but this has come at the expense of reproducibility. In this context, fields like organic photocatalysis and materials synthesis have also been affected. This Perspective aims at providing general guidelines to increase trustworthiness and favor reproducibility for those interdisciplinary researchers working on organic photocatalytic transformations catalyzed by carbon-nitride-based materials. Thus, the article focuses on the importance of accurately reporting and describing all the stages of experimental work, from the photocatalyst synthesis and characterization to the evaluation of the reaction conditions, control experiments, and─more generally─all the details that may ensure reproducibility. Additionally, we investigate and discuss the risks of falling into inadequate research practices, emphasizing that irreproducibility in science is a major problem that undermines the utility and credibility of scientific research. These aspects are crucial for the scientific community, and we emphasize the need to raise awareness and educate researchers toward best experimental practices.

Abstract Image

氮化碳有机光催化的可靠和可重复性研究
在过去的几十年里,科学出版物的速度呈指数级增长,但这是以可重复性为代价的。在此背景下,有机光催化和材料合成等领域也受到了影响。本展望旨在为从事碳氮基材料催化的有机光催化转化的跨学科研究人员提供提高可靠性和可重复性的一般指南。因此,本文着重于准确报告和描述实验工作的所有阶段的重要性,从光催化剂的合成和表征到反应条件的评估,控制实验,以及更一般地说,所有可能确保再现性的细节。此外,我们调查和讨论了陷入不充分的研究实践的风险,强调科学中的不可重复性是破坏科学研究的效用和可信度的主要问题。这些方面对科学界至关重要,我们强调需要提高认识并教育研究人员进行最佳实验实践。
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来源期刊
ACS Catalysis
ACS Catalysis CHEMISTRY, PHYSICAL-
CiteScore
20.80
自引率
6.20%
发文量
1253
审稿时长
1.5 months
期刊介绍: ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels. The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.
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