Single photon superradiance enhanced light–matter interaction in spatially ordered shape and volume controlled single quantum dots: enabling on-chip photonic networks

IF 6.6 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Lucas Jordao, Swarnabha Chattaraj, Qi Huang, Siyuan Lu, Jiefei Zhang, Anupam Madhukar
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Abstract

On-chip photonic networks require adequately spatially ordered matter-photon interconversion qubit sources with emission figures-of-merit exceeding the requirements that would enable the desired functional response of the network. The mesa-top single quantum dots (MTSQDs) have recently been demonstrated to meet these requirements. The substrate-encoded size-reducing epitaxy (SESRE) approach underpinning the realization of these unique quantum emitters allows control on the shape, size, and strain (lattice-matched or mismatched) of these epitaxial single quantum dots. We have exploited this unique feature of the MTSQDs to reproducibly create arrays of quantum dots that exhibit single photon superradiance, a characteristic of the SESRE-enabled delicate balance between the confinement potential volume, depth, the resulting exciton binding energy, and the degree of confinement of the center of mass (CM) motion of the exciton. Scanning transmission electron microscope (STEM) studies reveal the structural (atomic scale) and chemical (nanometer scale) nature of the material region defining the notion of the shape and volume (here large) of the electron confinement region (i.e. the QD). In the exciton’s weak CM confinement regime, owing to its coherent sampling of the large volume, an enhancement of the MTSQD oscillator strength to ∼30 is demonstrated. Theoretical modelling with input from the STEM findings provides corroboration for single photon superradiance causing enhancement of the oscillator strength by ∼2.5–3. Our findings allow fabricating and studying interconnected networks enabled by these unique matter qubit-light qubit interconversion units that can be realized for lattice matched and mismatched material combinations covering UV to mid-infrared wavelength range.
单光子超辐射增强了空间有序形状和体积控制的单量子点的光-物质相互作用:实现片上光子网络
片上光子网络需要足够的空间有序的物质-光子互转换量子比特源,其发射值超过了能够实现网络所需功能响应的要求。台式单量子点(MTSQDs)最近被证明可以满足这些要求。衬底编码减小尺寸外延(SESRE)方法支持这些独特量子发射器的实现,允许控制这些外延单量子点的形状,大小和应变(晶格匹配或不匹配)。我们利用mtsqd的这一独特特性,可重复地创建具有单光子超辐射的量子点阵列,这是ssese支持的约束势体积、深度、产生的激子结合能和激子质心运动的限制程度之间的微妙平衡的特征。扫描透射电子显微镜(STEM)研究揭示了材料区域的结构(原子尺度)和化学(纳米尺度)性质,定义了电子约束区域(即QD)的形状和体积(这里是大的)的概念。在激子的弱CM约束状态下,由于其大体积的相干采样,MTSQD振荡器强度增强到~ 30。从STEM研究结果输入的理论建模证实了单光子超辐射导致振荡器强度增强约2.5-3。我们的发现允许制造和研究由这些独特的物质量子比特-光量子比特相互转换单元实现的互联网络,这些单元可以实现晶格匹配和不匹配的材料组合,覆盖紫外线到中红外波长范围。
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来源期刊
Nanophotonics
Nanophotonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
13.50
自引率
6.70%
发文量
358
审稿时长
7 weeks
期刊介绍: Nanophotonics, published in collaboration with Sciencewise, is a prestigious journal that showcases recent international research results, notable advancements in the field, and innovative applications. It is regarded as one of the leading publications in the realm of nanophotonics and encompasses a range of article types including research articles, selectively invited reviews, letters, and perspectives. The journal specifically delves into the study of photon interaction with nano-structures, such as carbon nano-tubes, nano metal particles, nano crystals, semiconductor nano dots, photonic crystals, tissue, and DNA. It offers comprehensive coverage of the most up-to-date discoveries, making it an essential resource for physicists, engineers, and material scientists.
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