InSe-Based Sensors and Related Sensing Systems for NO2 Gas/Temperature Monitoring

IF 9.1 1区 化学 Q1 CHEMISTRY, ANALYTICAL
Mingyang Gao, , , Bohang Zhang, , , Xinyuan Du, , , Xueqian Yang, , , Chunxue Zhai, , , Cheng Chen*, , , Zhiyong Zhang, , and , Wu Zhao*, 
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Abstract

High-sensitivity, multiparameter sensing is increasingly critical for environmental monitoring and electronics. Existing sensing platforms struggle to integrate precise, rapid, and stable monitoring of parts per billion-level hazardous gases and temperature within a single miniaturized device. This study developed a novel sensor based on two-dimensional (2D) indium selenide (InSe), complemented by first-principles density functional theory calculations elucidating the layer-dependent NO2 adsorption mechanism. The sensor demonstrated exceptional dual-mode performance, achieving a 103.40% response to 2 ppm of NO2 alongside a broad temperature detection range (25–150 °C) with high sensitivity. To enable practical applications, we further integrated the sensor into a portable intelligent monitoring system that features signal acquisition, processing, and alarm. This integrated bifunctional platform significantly advances miniaturized, multiparameter sensing technology, offering a powerful solution for next-generation environmental monitors and devices.

Abstract Image

用于NO2气体/温度监测的基于inse的传感器和相关传感系统。
高灵敏度、多参数传感在环境监测和电子领域日益重要。现有的传感平台难以在单个小型化设备中集成精确、快速和稳定的十亿分之一级别有害气体和温度监测。本研究开发了一种基于二维(2D)硒化铟(InSe)的新型传感器,并辅以第一性原理密度泛函理论计算,阐明了依赖于层的NO2吸附机理。该传感器具有出色的双模性能,对2 ppm NO2的响应达到103.40%,同时具有高灵敏度的宽温度检测范围(25-150°C)。为了实现实际应用,我们进一步将传感器集成到具有信号采集,处理和报警功能的便携式智能监控系统中。这种集成的双功能平台显著推进了小型化、多参数传感技术,为下一代环境监测仪和设备提供了强大的解决方案。
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来源期刊
ACS Sensors
ACS Sensors Chemical Engineering-Bioengineering
CiteScore
14.50
自引率
3.40%
发文量
372
期刊介绍: ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.
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