{"title":"Impact of oil and gas emissions on summertime air quality in the Northern Great Plains: WRF-Chem modeling analysis","authors":"Carlos J. Bucaram , Frank M. Bowman","doi":"10.1016/j.atmosenv.2025.121509","DOIUrl":null,"url":null,"abstract":"<div><div>Oil and gas production increased dramatically last decade in the Bakken region, with accompanying changes to pollutant emissions and atmospheric concentrations. WRF-Chem model simulations of the Northern Great Plains were conducted comparing two emission scenarios using 2011 emissions to represent a baseline case with relatively low oil production (<0.4 million barrels per day) and 2014 emissions to represent a high production case (> 1.0 million barrels per day). Assessment of model predictions from the baseline scenario against ground level meteorology and air quality measurements showed good overall agreement, demonstrating suitable model performance for assessing the effect of emissions changes on pollutant levels. In the high production scenario emissions of SO<sub>2</sub> and NO<sub>x</sub> were lower across most of the domain (-80% and -37%, respectively), but were significantly higher in the Bakken region (+62% for SO<sub>2</sub> and +110% for NO<sub>x</sub>), and changes in VOC emissions were also relatively higher in the Bakken. Simulated pollutant concentrations followed these emission changes, with average NO<sub>x</sub> levels decreasing for the high production scenario by 22% in the overall domain, but increasing by 72% in the Bakken. Predicted average O<sub>3</sub> levels increased slightly by 0.2% across the domain as NO<sub>x</sub> levels decreased, characteristic of VOC-limited conditions, with larger increases in urban areas where NO<sub>x</sub> reductions were greater. For the Bakken, simulations predict localized O<sub>3</sub> decreases in the center of the region, but increases in downwind areas. Changes between the baseline and high production scenarios demonstrate the influence of oil and gas production associated emissions on pollutant concentrations.</div></div>","PeriodicalId":250,"journal":{"name":"Atmospheric Environment","volume":"361 ","pages":"Article 121509"},"PeriodicalIF":3.7000,"publicationDate":"2025-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Environment","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1352231025004844","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0
Abstract
Oil and gas production increased dramatically last decade in the Bakken region, with accompanying changes to pollutant emissions and atmospheric concentrations. WRF-Chem model simulations of the Northern Great Plains were conducted comparing two emission scenarios using 2011 emissions to represent a baseline case with relatively low oil production (<0.4 million barrels per day) and 2014 emissions to represent a high production case (> 1.0 million barrels per day). Assessment of model predictions from the baseline scenario against ground level meteorology and air quality measurements showed good overall agreement, demonstrating suitable model performance for assessing the effect of emissions changes on pollutant levels. In the high production scenario emissions of SO2 and NOx were lower across most of the domain (-80% and -37%, respectively), but were significantly higher in the Bakken region (+62% for SO2 and +110% for NOx), and changes in VOC emissions were also relatively higher in the Bakken. Simulated pollutant concentrations followed these emission changes, with average NOx levels decreasing for the high production scenario by 22% in the overall domain, but increasing by 72% in the Bakken. Predicted average O3 levels increased slightly by 0.2% across the domain as NOx levels decreased, characteristic of VOC-limited conditions, with larger increases in urban areas where NOx reductions were greater. For the Bakken, simulations predict localized O3 decreases in the center of the region, but increases in downwind areas. Changes between the baseline and high production scenarios demonstrate the influence of oil and gas production associated emissions on pollutant concentrations.
期刊介绍:
Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.