Impact of oil and gas emissions on summertime air quality in the Northern Great Plains: WRF-Chem modeling analysis

IF 3.7 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Carlos J. Bucaram , Frank M. Bowman
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Abstract

Oil and gas production increased dramatically last decade in the Bakken region, with accompanying changes to pollutant emissions and atmospheric concentrations. WRF-Chem model simulations of the Northern Great Plains were conducted comparing two emission scenarios using 2011 emissions to represent a baseline case with relatively low oil production (<0.4 million barrels per day) and 2014 emissions to represent a high production case (> 1.0 million barrels per day). Assessment of model predictions from the baseline scenario against ground level meteorology and air quality measurements showed good overall agreement, demonstrating suitable model performance for assessing the effect of emissions changes on pollutant levels. In the high production scenario emissions of SO2 and NOx were lower across most of the domain (-80% and -37%, respectively), but were significantly higher in the Bakken region (+62% for SO2 and +110% for NOx), and changes in VOC emissions were also relatively higher in the Bakken. Simulated pollutant concentrations followed these emission changes, with average NOx levels decreasing for the high production scenario by 22% in the overall domain, but increasing by 72% in the Bakken. Predicted average O3 levels increased slightly by 0.2% across the domain as NOx levels decreased, characteristic of VOC-limited conditions, with larger increases in urban areas where NOx reductions were greater. For the Bakken, simulations predict localized O3 decreases in the center of the region, but increases in downwind areas. Changes between the baseline and high production scenarios demonstrate the influence of oil and gas production associated emissions on pollutant concentrations.
石油和天然气排放对北部大平原夏季空气质量的影响:WRF-Chem模型分析
在过去的十年中,Bakken地区的石油和天然气产量急剧增加,随之而来的是污染物排放和大气浓度的变化。WRF-Chem模型对北部大平原进行了两种排放情景的模拟,其中2011年的排放量代表了相对较低的石油产量(40万桶/天)的基线情况,2014年的排放量代表了较高的产量情况(100万桶/天)。根据地面气象学和空气质量测量结果对基线情景的模式预测进行评估,结果显示出良好的总体一致性,表明模式在评估排放变化对污染物水平的影响方面表现合适。在高产量情景下,大部分地区的SO2和NOx排放量较低(分别为-80%和-37%),但在巴肯地区明显较高(SO2为+62%,NOx为+110%),并且巴肯地区VOC排放量的变化也相对较高。模拟污染物浓度随排放变化而变化,在整个区域,高产量情景的平均氮氧化物水平下降了22%,但在巴肯地区,平均氮氧化物水平上升了72%。随着氮氧化物水平的下降,预测的平均O3水平在整个区域内略有上升0.2%,这是voc限制条件的特征,在氮氧化物减少幅度较大的城市地区,预测的平均O3水平上升幅度较大。对于巴肯,模拟预测该区域中心的局部O3会减少,但在下风区域会增加。基线情景和高产量情景之间的变化表明,油气生产相关排放对污染物浓度的影响。
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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