Preparation of coated fabrics with efficient radiation cooling and self-cleaning properties

IF 7.3 2区 材料科学 Q1 CHEMISTRY, APPLIED
Yijun Fu , Jiahao Yu , Zhongyuan Yuan , Mengdi Xue , Hongbin Lu , Song Chu , Wei Zhang , Dawei Li
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Abstract

Facing the challenges of global warming and increasing energy consumption, the development of new textile materials with efficient thermal management and self-cleaning functions has become crucial. In this study, a composite coated fabric consisting of polyvinylidene fluoride (PVDF), thermoplastic polyurethane (TPU) and nano‑silicon dioxide (SiO2) was successfully prepared by a scratch coating process. The experimental results show that the material exhibits high light reflectivity of 89 % in the visible band, while realizing excellent thermal radiation efficiency of 97.5 % in the mid-infrared band, and this dual-frequency synergy significantly reduced the average temperature of the fabric surface by 11.7 °C compared to the untreated sample. The maximum cooling efficiency reached 13.1 °C and the net radiative cooling power reaches ∼120 W/m2 demonstrating groundbreaking thermal management performance. Notably, through the optimization of the material ratio, the coated surface forms a remarkable superhydrophobic property with a water contact angle of 155 ± 1°, effectively realizing the self-cleaning function with a droplet rolling angle of less than 10°. Crucially, this approach achieves these outstanding radiative cooling and superhydrophobic properties while significantly enhancing the coating's adhesion to the fabric substrate. This multifunctionality allows the coated fabric to show great potential in outdoor tents, clothing and other thermal management applications, providing innovative solutions for combating climate change and resource conservation.
具有高效辐射冷却和自清洁性能的涂层织物的制备
面对全球变暖和能源消耗增加的挑战,开发具有高效热管理和自清洁功能的新型纺织材料变得至关重要。在本研究中,通过划痕涂层工艺成功制备了由聚偏氟乙烯(PVDF)、热塑性聚氨酯(TPU)和纳米二氧化硅(SiO2)组成的复合涂层织物。实验结果表明,该材料在可见光波段具有89%的高反射率,而在中红外波段具有97.5%的优异热辐射效率,并且这种双频协同作用显著降低了织物表面的平均温度,比未处理的样品降低了11.7℃。最高冷却效率达到13.1°C,净辐射冷却功率达到~ 120 W/m2,展示了突破性的热管理性能。值得注意的是,通过优化材料配比,涂层表面形成了显著的超疏水性,水接触角为155±1°,有效实现了液滴滚动角小于10°的自清洁功能。至关重要的是,这种方法实现了这些出色的辐射冷却和超疏水性,同时显著提高了涂层与织物基底的附着力。这种多功能使得涂层织物在户外帐篷、服装和其他热管理应用中显示出巨大的潜力,为应对气候变化和资源保护提供了创新的解决方案。
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来源期刊
Progress in Organic Coatings
Progress in Organic Coatings 工程技术-材料科学:膜
CiteScore
11.40
自引率
15.20%
发文量
577
审稿时长
48 days
期刊介绍: The aim of this international journal is to analyse and publicise the progress and current state of knowledge in the field of organic coatings and related materials. The Editors and the Editorial Board members will solicit both review and research papers from academic and industrial scientists who are actively engaged in research and development or, in the case of review papers, have extensive experience in the subject to be reviewed. Unsolicited manuscripts will be accepted if they meet the journal''s requirements. The journal publishes papers dealing with such subjects as: • Chemical, physical and technological properties of organic coatings and related materials • Problems and methods of preparation, manufacture and application of these materials • Performance, testing and analysis.
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