Man Yue , Yawen Liu , Minghuai Wang , Xinyi Dong , Jianping Guo , Yuwen Niu , Honghui Xu
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引用次数: 0
Abstract
Interactions between aerosols and the planetary boundary layer (PBL) play a crucial role in aggravating air quality and modulating regional climate. Despite intensive studies exploring the aerosol-PBL interaction predominantly focused on short-term haze events, uncertainties remain in understanding this interaction over longer timescales. To fill this gap, we investigate the long-term trends of extremely high and low PBL height (PBLH) across China, utilizing multi-observed datasets and sensitivity experiments conducted with the Community Atmosphere Model version 6 (CAM6) with full chemistry. Here the extremely high (low) PBLH is defined as mean values of the daily PBLH higher (lower) than 90th (10th) percentile for each season. Our analysis reveals a significant increase in extremely high PBLH during the period 1979–2003 (seasonal ranging from +283.36 to +326.80 m/decade), followed by a pronounced reversal to declining trends during 2004–2016 (−321.45 to −178.83 m/decade). The trend shift is primarily driven by variations in surface sensible heat fluxes. Conversely, extremely low PBLH exhibits an obvious “negative to positive” trend shift around 2007 during 2000–2016, especially over Eastern and Central China (ECC) with a mean trend magnitude of +153.2 m/decade after 2007. The long-term trend of extremely low PBLH is dominated by changes in shortwave atmosphere absorption, which are influenced by the direct radiative effect of black carbon (BC) aerosols. Comparative simulations with BC's direct radiative effect turning on/off further demonstrate the reduced BC aerosols after 2007 diminishes the shortwave atmosphere absorption and enhances the surface shortwave radiation, thereby promoting an increase in extremely low PBLH, and vice versa. These findings highlight the distinct mechanisms influencing the long-term trend of extremely high and low PBLH over China, and provide new insights into the long-term variability of PBLH and its relationship with aerosols.
期刊介绍:
The journal publishes scientific papers (research papers, review articles, letters and notes) dealing with the part of the atmosphere where meteorological events occur. Attention is given to all processes extending from the earth surface to the tropopause, but special emphasis continues to be devoted to the physics of clouds, mesoscale meteorology and air pollution, i.e. atmospheric aerosols; microphysical processes; cloud dynamics and thermodynamics; numerical simulation, climatology, climate change and weather modification.