Danielle Land*, Grant D. Brown, David M. Cwiertny, Marc A. Edwards, Mona Hanna, Drew E. Latta and Michelle M. Scherer,
{"title":"A Novel, Metal-Based Approach to Identify Residences with Lead Service Lines","authors":"Danielle Land*, Grant D. Brown, David M. Cwiertny, Marc A. Edwards, Mona Hanna, Drew E. Latta and Michelle M. Scherer, ","doi":"10.1021/acs.estlett.5c00552","DOIUrl":null,"url":null,"abstract":"<p >There is an urgent need for rapid, cost-effective approaches to identify residences with lead service lines (LSLs). We evaluated whether analyzing water for corrosion-related metals could accurately identify residences with LSLs without relying on potentially inaccurate property records. We applied principal component analysis logistic regression (PCA-LR) and classification tree models using 28 analytes per bottle (including Pb, Cu, Zn, Fe, Al, and others) measured in 216 water samples collected in Flint, Michigan, in August 2015. The PCA-LR model achieved 87% accuracy (AUROC = 0.93) with 81% sensitivity and 90% specificity, while the classification tree model achieved 80% accuracy (AUROC = 0.77) with 74% sensitivity and 84% specificity. The classification tree provided interpretable decision rules identifying key predictive metals, primarily relying on 1 min flush Pb concentrations with Zn and Al as secondary predictors. It also revealed distinct metal co-occurrence patterns between LSLs and premise plumbing, offering insights into Pb source identification. The tree’s interpretable structure makes it particularly valuable for practical implementation by utilities. Although additional work is needed to extend these models to other water systems, our results suggest that metal analysis provides an accurate, cost-effective, and minimally invasive tool that complements existing approaches for predicting the presence of an LSL.</p>","PeriodicalId":37,"journal":{"name":"Environmental Science & Technology Letters Environ.","volume":"12 8","pages":"918–923"},"PeriodicalIF":8.8000,"publicationDate":"2025-07-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acs.estlett.5c00552","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science & Technology Letters Environ.","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.estlett.5c00552","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0
Abstract
There is an urgent need for rapid, cost-effective approaches to identify residences with lead service lines (LSLs). We evaluated whether analyzing water for corrosion-related metals could accurately identify residences with LSLs without relying on potentially inaccurate property records. We applied principal component analysis logistic regression (PCA-LR) and classification tree models using 28 analytes per bottle (including Pb, Cu, Zn, Fe, Al, and others) measured in 216 water samples collected in Flint, Michigan, in August 2015. The PCA-LR model achieved 87% accuracy (AUROC = 0.93) with 81% sensitivity and 90% specificity, while the classification tree model achieved 80% accuracy (AUROC = 0.77) with 74% sensitivity and 84% specificity. The classification tree provided interpretable decision rules identifying key predictive metals, primarily relying on 1 min flush Pb concentrations with Zn and Al as secondary predictors. It also revealed distinct metal co-occurrence patterns between LSLs and premise plumbing, offering insights into Pb source identification. The tree’s interpretable structure makes it particularly valuable for practical implementation by utilities. Although additional work is needed to extend these models to other water systems, our results suggest that metal analysis provides an accurate, cost-effective, and minimally invasive tool that complements existing approaches for predicting the presence of an LSL.
期刊介绍:
Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.