{"title":"Ultrabroadband nonlinear Hall rectifier using SnTe","authors":"Fanrui Hu, Pengnan Zhao, Lihuan Yang, Shishun Zhao, Jiayu Lei, Weijian Li, Jiamin Lai, Zhonghai Yu, Hanbum Park, Chengquan Wong, Raghav Sharma, Goki Eda, Shengyuan A. Yang, Xiaohong Xu, Fei Wang, Hyunsoo Yang","doi":"10.1038/s41565-025-01993-2","DOIUrl":null,"url":null,"abstract":"<p>The rapid expansion of self-powered electronics in the Internet of Things, 6G communication and millimetre-wave systems calls for rectifiers capable of operating across ultrabroadband frequencies and at extremely low input power levels. However, conventional rectifiers based on semiconductor junctions face fundamental limitations such as parasitic capacitance and threshold voltages, preventing effective operation under broadband and ambient radio-frequency conditions. Here we present an ultrabroadband, zero-bias rectifier based on the nonlinear Hall effect in wafer-scale (001)-oriented topological crystalline insulator SnTe thin film. This material exhibits a large second-order conductivity of ~0.004 Ω⁻<sup>1</sup> V⁻<sup>1</sup>, surpassing that of other wafer-scale materials. The nonlinear Hall effect arises primarily from a Berry curvature dipole, evidenced by angular-resolved transport measurements and first-principles calculations. The device demonstrates rectification from 23 MHz to 1 THz, with sensitivity down to –60 dBm in key radio-frequency bands, without any external bias. Rectified output power is scalable through series- and parallel-array topologies and can be enhanced using rectenna designs. As a proof of concept, we achieve the wireless powering of a thermistor using harvested radio-frequency energy, validating the potential of this material platform and nonlinear Hall effect for next-generation energy-autonomous microsystems.</p>","PeriodicalId":18915,"journal":{"name":"Nature nanotechnology","volume":"8 1","pages":""},"PeriodicalIF":34.9000,"publicationDate":"2025-08-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature nanotechnology","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41565-025-01993-2","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The rapid expansion of self-powered electronics in the Internet of Things, 6G communication and millimetre-wave systems calls for rectifiers capable of operating across ultrabroadband frequencies and at extremely low input power levels. However, conventional rectifiers based on semiconductor junctions face fundamental limitations such as parasitic capacitance and threshold voltages, preventing effective operation under broadband and ambient radio-frequency conditions. Here we present an ultrabroadband, zero-bias rectifier based on the nonlinear Hall effect in wafer-scale (001)-oriented topological crystalline insulator SnTe thin film. This material exhibits a large second-order conductivity of ~0.004 Ω⁻1 V⁻1, surpassing that of other wafer-scale materials. The nonlinear Hall effect arises primarily from a Berry curvature dipole, evidenced by angular-resolved transport measurements and first-principles calculations. The device demonstrates rectification from 23 MHz to 1 THz, with sensitivity down to –60 dBm in key radio-frequency bands, without any external bias. Rectified output power is scalable through series- and parallel-array topologies and can be enhanced using rectenna designs. As a proof of concept, we achieve the wireless powering of a thermistor using harvested radio-frequency energy, validating the potential of this material platform and nonlinear Hall effect for next-generation energy-autonomous microsystems.
期刊介绍:
Nature Nanotechnology is a prestigious journal that publishes high-quality papers in various areas of nanoscience and nanotechnology. The journal focuses on the design, characterization, and production of structures, devices, and systems that manipulate and control materials at atomic, molecular, and macromolecular scales. It encompasses both bottom-up and top-down approaches, as well as their combinations.
Furthermore, Nature Nanotechnology fosters the exchange of ideas among researchers from diverse disciplines such as chemistry, physics, material science, biomedical research, engineering, and more. It promotes collaboration at the forefront of this multidisciplinary field. The journal covers a wide range of topics, from fundamental research in physics, chemistry, and biology, including computational work and simulations, to the development of innovative devices and technologies for various industrial sectors such as information technology, medicine, manufacturing, high-performance materials, energy, and environmental technologies. It includes coverage of organic, inorganic, and hybrid materials.