Reconfigurable Tin-Halide Perovskite Resistive Switching Memory for Reservoir Computing System in Braille Code Translator

IF 8.7 1区 化学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Dohyung Kim, Hansol Park and Hui Joon Park*, 
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引用次数: 0

Abstract

Resistive switching memories (RSMs) have emerged as promising candidates for a reservoir computing (RC) system, which excels in processing temporal information. Their ability to function as either volatile or nonvolatile devices makes them ideal for reservoir and readout layers. However, conventional RSMs require separate devices for these functionalities, complicating integrated RC systems. Here, we introduce tin-halide perovskite as a switching medium and present a reconfigurable RSM with Pt/FASnI3/Ag structure that integrates volatile and nonvolatile properties by modulating switching mechanisms. Under a positive bias to the Pt electrode, the device operates in a volatile threshold-switching mode based on space-charge-limited conduction, exhibiting short-term dynamics─key features for reservoir layers. On the other hand, applying positive bias to the Ag electrode activates a nonvolatile bipolar-switching mode, driven by reversible filamentary mechanisms, with long-term potentiation and depression characteristics, suitable for readout layers. Using this reconfigurable RSM, we developed a hardware RC system for Braille code recognition.

Abstract Image

用于盲文翻译器储层计算系统的可重构锡卤化钙钛矿电阻开关存储器
电阻开关存储器(RSMs)在处理时间信息方面表现优异,是储层计算(RC)系统的一个有希望的候选者。它们作为挥发性或非挥发性器件的功能使其成为储层和读出层的理想选择。然而,传统的rsm需要单独的设备来实现这些功能,使集成RC系统复杂化。在这里,我们引入了卤化锡钙钛矿作为开关介质,并提出了一种具有Pt/FASnI3/Ag结构的可重构RSM,该结构通过调制开关机制集成了易失性和非易失性。在Pt电极的正偏压下,该器件以基于空间电荷限制传导的挥发性阈值开关模式工作,表现出短期动力学──储层的关键特征。另一方面,在Ag电极上施加正偏压可激活由可逆丝状机制驱动的非易失性双极开关模式,具有长期增强和抑制特性,适合于读出层。利用这种可重构RSM,我们开发了一个用于盲文识别的硬件RSM系统。
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来源期刊
ACS Materials Letters
ACS Materials Letters MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
14.60
自引率
3.50%
发文量
261
期刊介绍: ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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