The Role of Wind Velocity in Saline Water Evaporation from Porous Media and Surface Salt Crystallization Dynamics

IF 2.9 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Sahar Jannesarahmadi*, Milad Aminzadeh*, Rainer Helmig, Dani Or, Bastian Oesterle and Nima Shokri*, 
{"title":"The Role of Wind Velocity in Saline Water Evaporation from Porous Media and Surface Salt Crystallization Dynamics","authors":"Sahar Jannesarahmadi*,&nbsp;Milad Aminzadeh*,&nbsp;Rainer Helmig,&nbsp;Dani Or,&nbsp;Bastian Oesterle and Nima Shokri*,&nbsp;","doi":"10.1021/acsearthspacechem.5c00130","DOIUrl":null,"url":null,"abstract":"<p >This study systematically investigates the effect of wind flow on evaporation dynamics and salt crystallization patterns in porous media. Well-controlled experiments were conducted in a laboratory wind tunnel, where the surface of sand columns saturated with freshwater and NaCl solutions at concentrations of 10%, 15%, and 20% were subjected to wind flows of 0.5 and 5 m/s, corresponding to laminar and turbulent flow regimes, respectively. Mass loss measurements from the samples, combined with optical imaging of their surfaces, revealed distinct evaporation dynamics and crystallization patterns. We observed that the interaction between intermittent turbulent airflow and evolving salt crystals on the surface resulted in a relatively uniform crystallization pattern. In contrast, under laminar airflow conditions, salt crystal nucleation and formation primarily occurred at the leading edge of the sample, particularly at lower salt concentrations. We further investigated the impact of enhanced evaporative mass loss in the presence of wind on crystallization dynamics by quantifying the crystal coverage and its lateral extent on the surface. Under turbulent flow conditions, we observed that full coverage of the surface with salt crystals requires 2 to 3 times higher evaporative losses in 10% NaCl sample relative to the 15% and 20% samples, respectively. These findings highlight the complex interplay between evaporation and crystallization processes under varying airflow conditions, thus offering valuable insight for improving hydrological and climatological modeling.</p>","PeriodicalId":15,"journal":{"name":"ACS Earth and Space Chemistry","volume":"9 7","pages":"1938–1945"},"PeriodicalIF":2.9000,"publicationDate":"2025-07-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsearthspacechem.5c00130","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Earth and Space Chemistry","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsearthspacechem.5c00130","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

This study systematically investigates the effect of wind flow on evaporation dynamics and salt crystallization patterns in porous media. Well-controlled experiments were conducted in a laboratory wind tunnel, where the surface of sand columns saturated with freshwater and NaCl solutions at concentrations of 10%, 15%, and 20% were subjected to wind flows of 0.5 and 5 m/s, corresponding to laminar and turbulent flow regimes, respectively. Mass loss measurements from the samples, combined with optical imaging of their surfaces, revealed distinct evaporation dynamics and crystallization patterns. We observed that the interaction between intermittent turbulent airflow and evolving salt crystals on the surface resulted in a relatively uniform crystallization pattern. In contrast, under laminar airflow conditions, salt crystal nucleation and formation primarily occurred at the leading edge of the sample, particularly at lower salt concentrations. We further investigated the impact of enhanced evaporative mass loss in the presence of wind on crystallization dynamics by quantifying the crystal coverage and its lateral extent on the surface. Under turbulent flow conditions, we observed that full coverage of the surface with salt crystals requires 2 to 3 times higher evaporative losses in 10% NaCl sample relative to the 15% and 20% samples, respectively. These findings highlight the complex interplay between evaporation and crystallization processes under varying airflow conditions, thus offering valuable insight for improving hydrological and climatological modeling.

风速对多孔介质中盐水蒸发及表面盐结晶动力学的影响
本研究系统地研究了气流对多孔介质中蒸发动力学和盐结晶模式的影响。在实验室风洞中进行了控制良好的实验,将饱和浓度分别为10%、15%和20%的淡水和NaCl溶液的砂柱表面分别置于0.5和5 m/s的气流中,分别对应于层流和湍流。样品的质量损失测量,结合其表面的光学成像,揭示了不同的蒸发动力学和结晶模式。我们观察到间歇性湍流气流与表面盐晶体演化的相互作用导致了相对均匀的结晶模式。相反,在层流条件下,盐晶体的成核和形成主要发生在样品的前缘,特别是在低盐浓度下。我们进一步研究了在风的作用下蒸发质量损失的增加对结晶动力学的影响,通过量化晶体覆盖及其在表面的横向范围。在湍流条件下,我们观察到,在10% NaCl样品中,盐晶体完全覆盖表面所需的蒸发损失分别是15%和20% NaCl样品的2 ~ 3倍。这些发现突出了在不同气流条件下蒸发和结晶过程之间复杂的相互作用,从而为改进水文和气候学模型提供了有价值的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
ACS Earth and Space Chemistry
ACS Earth and Space Chemistry Earth and Planetary Sciences-Geochemistry and Petrology
CiteScore
5.30
自引率
11.80%
发文量
249
期刊介绍: The scope of ACS Earth and Space Chemistry includes the application of analytical, experimental and theoretical chemistry to investigate research questions relevant to the Earth and Space. The journal encompasses the highly interdisciplinary nature of research in this area, while emphasizing chemistry and chemical research tools as the unifying theme. The journal publishes broadly in the domains of high- and low-temperature geochemistry, atmospheric chemistry, marine chemistry, planetary chemistry, astrochemistry, and analytical geochemistry. ACS Earth and Space Chemistry publishes Articles, Letters, Reviews, and Features to provide flexible formats to readily communicate all aspects of research in these fields.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信