Experimental study of onboard carbon capture pilot plant with a compact integrated stripper under variable parameters

IF 10 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Yijiang Tian, Zhen Tian, Wenzhong Gao, Yihang Zhou, Yuan Zhang, Xi Jin, Pelin Bolat, Yibo Zhou, Xikang Wang
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Abstract

In this paper, a new compact onboard carbon capture system (COCCS) for ships was proposed. The system had a reboiler and stripper as a single unit, and the structure of built-in coils provided a method for the utilization of ship flue gas waste heat. A parametric study was conducted to improve the operational efficiency of the COCCS. Emphasis was placed on reducing the energy consumption by changing the parameters only, without increasing system construction costs. Therefore, a COCCS pilot plant was established to obtain the database for multi-parameter testing. The parameters were designed according to the actual gas emissions from the ship, where the flue gas input concentration was 4–10 %, and the liquid-to-gas ratio (L/G) was 2–6. The desorption pressure (1.1–2.1 bar) was adjusted to give a large improvement in the system performance with "a lossless gain characteristic". The experimental results showed that the highest capture efficiency of 88.6 %, the lowest regeneration heat of 3.97 MJ/kgCO2, and the highest recycle capacity of 0.27 mol/mol were achieved under parameter optimization. The optimization of L/G showed the most significant improvement in the capture efficiency, which was enhanced by 15.06 %. The optimization of desorption pressure showed the most significant improvement in regeneration heat with a reduction of 44 %. This study provided support for parameter schemes for existing and future onboard carbon capture devices and highlighted the potential for parameter optimization to improve system performance without additional infrastructure investment.
变参数下小型集成汽提器机载碳捕集中试装置的实验研究
提出了一种新型紧凑型船用碳捕集系统。该系统以再沸器和汽提塔为一体,内置盘管的结构为船舶烟气余热的利用提供了一种方法。为了提高系统的运行效率,进行了参数化研究。重点是通过改变参数来降低能耗,而不增加系统建设成本。为此,建立了一个caccs中试装置,以获取多参数测试数据库。根据船舶实际烟气排放情况进行参数设计,烟气输入浓度为4 ~ 10%,液气比(L/G)为2 ~ 6。通过调整解吸压力(1.1-2.1 bar),系统性能得到了很大的改善,具有“无损增益特性”。实验结果表明,经参数优化后,捕集效率最高为88.6%,再生热最低为3.97 MJ/kgCO2,再生容量最高为0.27 mol/mol。L/G优化对捕集效率的提高最为显著,提高了15.06%。优化后的脱附压力对再生热的改善最为显著,降低了44%。该研究为现有和未来车载碳捕获设备的参数方案提供了支持,并强调了参数优化的潜力,以提高系统性能,而无需额外的基础设施投资。
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来源期刊
Journal of Cleaner Production
Journal of Cleaner Production 环境科学-工程:环境
CiteScore
20.40
自引率
9.00%
发文量
4720
审稿时长
111 days
期刊介绍: The Journal of Cleaner Production is an international, transdisciplinary journal that addresses and discusses theoretical and practical Cleaner Production, Environmental, and Sustainability issues. It aims to help societies become more sustainable by focusing on the concept of 'Cleaner Production', which aims at preventing waste production and increasing efficiencies in energy, water, resources, and human capital use. The journal serves as a platform for corporations, governments, education institutions, regions, and societies to engage in discussions and research related to Cleaner Production, environmental, and sustainability practices.
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