Research progress and perspectives on rechargeable batteries

IF 8.9 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Chinese Chemical Letters Pub Date : 2025-04-08 DOI:10.1016/j.cclet.2025.111185

Gaojing Yang , Zhimeng Hao , Chun Fang , Wen Zhang , Xia-hui Zhang , Yuyu Li , Zhenhua Yan , Zhiyuan Wang , Tao Sun , Xiaofei Yang , Fei Wang , Chengzhi Zhang , Hongchang Jin , Shuaifeng Lou , Nan Chen , Yiju Li , Jia-Yan Liang , Le Yang , Shouyi Yuan , Jin Niu , Jianmin Ma

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Abstract

Energy storage plays a critical role in sustainable development, with secondary batteries serving as vital technologies for efficient energy conversion and utilization. This review provides a comprehensive summary of recent advancements across various battery systems, including lithium-ion, sodium-ion, potassium-ion, and multivalent metal-ion batteries such as magnesium, zinc, calcium, and aluminum. Emerging technologies, including dual-ion, redox flow, and anion batteries, are also discussed. Particular attention is given to alkali metal rechargeable systems, such as lithium-sulfur, lithium-air, sodium-sulfur, sodium-selenium, potassium-sulfur, potassium-selenium, potassium-air, and zinc-air batteries, which have shown significant promise for high-energy applications. The optimization of key components—cathodes, anodes, electrolytes, and interfaces—is extensively analyzed, supported by advanced characterization techniques like time-of-flight secondary ion mass spectrometry (TOF-SIMS), synchrotron radiation, nuclear magnetic resonance (NMR), and in-situ spectroscopy. Moreover, sustainable strategies for recycling spent batteries, including pyrometallurgy, hydrometallurgy, and direct recycling, are critically evaluated to mitigate environmental impacts and resource scarcity. This review not only highlights the latest technological breakthroughs but also identifies key challenges in reaction mechanisms, material design, system integration, and waste battery recycling, and presents a roadmap for advancing high-performance and sustainable battery technologies.

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可充电电池的研究进展与展望

能源储存在可持续发展中起着至关重要的作用，而二次电池是实现能源高效转换和利用的重要技术。本文综述了各种电池系统的最新进展，包括锂离子、钠离子、钾离子和多价金属离子电池，如镁、锌、钙和铝。新兴技术，包括双离子，氧化还原流和阴离子电池，也进行了讨论。特别关注碱金属可充电系统，如锂-硫电池、锂-空气电池、钠-硫电池、钠-硒电池、钾-硫电池、钾-硒电池、钾-空气电池和锌-空气电池，它们在高能应用中显示出巨大的前景。通过先进的表征技术，如飞行时间二次离子质谱（TOF-SIMS）、同步辐射、核磁共振（NMR）和原位光谱学，对阴极、阳极、电解质和界面等关键部件的优化进行了广泛的分析。此外，对回收废电池的可持续战略，包括火法冶金、湿法冶金和直接回收，进行了严格评估，以减轻环境影响和资源稀缺。本文不仅强调了最新的技术突破，而且指出了在反应机理、材料设计、系统集成和废电池回收等方面的关键挑战，并提出了推进高性能和可持续电池技术的路线图。

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来源期刊

Chinese Chemical Letters 化学-化学综合

CiteScore

14.10

自引率

15.40%

发文量

8969

审稿时长

1.6 months

期刊介绍： Chinese Chemical Letters (CCL) (ISSN 1001-8417) was founded in July 1990. The journal publishes preliminary accounts in the whole field of chemistry, including inorganic chemistry, organic chemistry, analytical chemistry, physical chemistry, polymer chemistry, applied chemistry, etc.Chinese Chemical Letters does not accept articles previously published or scheduled to be published. To verify originality, your article may be checked by the originality detection service CrossCheck.