Real-time observation of topological defect dynamics mediating two-dimensional skyrmion lattice melting

IF 34.9 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Raphael Gruber, Jan Rothörl, Simon M. Fröhlich, Maarten A. Brems, Fabian Kammerbauer, Maria-Andromachi Syskaki, Elizabeth M. Jefremovas, Sachin Krishnia, Asle Sudbø, Peter Virnau, Mathias Kläui
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Abstract

Topological defects are the key feature mediating two-dimensional phase transitions. However, both resolution and tunability have been lacking to access the dynamics of these transitions in the various two-dimensional systems explored. Skyrmions in magnetic thin films are two-dimensional, topologically non-trivial quasi-particles that provide rich dynamics as well as tunability as an essential ingredient for the control of their phase behaviour. With dynamic Kerr microscopy, we directly capture the melting of a confined two-dimensional magnetic skyrmion lattice in a Ta/CoFeB/Ta/MgO/Ta magnetic multilayer system with high resolution in real time and real space. By the applied magnetic field, we tune the skyrmion size and effective temperature on the fly to drive the two-step melting through an intermediate hexatic regime between the solid lattice and the isotropic liquid. We quantify the characteristic occurrence of topological defects mediating the transitions and reveal the dynamics of the lattice dislocations. The full real-time and real-space imaging reveals the diffusion coefficient of dislocations, which is two orders of magnitude higher than that of skyrmions.

Abstract Image

二维skyrmion晶格熔化的拓扑缺陷动力学实时观察
拓扑缺陷是导致二维相变的关键特征。然而,在探索的各种二维系统中,分辨率和可调性都缺乏访问这些转变的动力学。磁薄膜中的Skyrmions是二维的,拓扑上非平凡的准粒子,提供丰富的动力学以及作为控制其相行为的基本成分的可调性。利用动态Kerr显微镜,我们实时、真实地捕捉到了Ta/CoFeB/Ta/MgO/Ta磁性多层体系中受限二维磁skyrmion晶格的熔化过程,并具有高分辨率。在外加磁场的作用下,通过调整粒子尺寸和有效温度来驱动固体晶格和各向同性液体之间的中间六向状态的两步熔化。我们量化了拓扑缺陷的特征发生,并揭示了晶格位错的动力学。全实时和实空间成像显示位错的扩散系数比skyrmions高两个数量级。
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来源期刊
Nature nanotechnology
Nature nanotechnology 工程技术-材料科学:综合
CiteScore
59.70
自引率
0.80%
发文量
196
审稿时长
4-8 weeks
期刊介绍: Nature Nanotechnology is a prestigious journal that publishes high-quality papers in various areas of nanoscience and nanotechnology. The journal focuses on the design, characterization, and production of structures, devices, and systems that manipulate and control materials at atomic, molecular, and macromolecular scales. It encompasses both bottom-up and top-down approaches, as well as their combinations. Furthermore, Nature Nanotechnology fosters the exchange of ideas among researchers from diverse disciplines such as chemistry, physics, material science, biomedical research, engineering, and more. It promotes collaboration at the forefront of this multidisciplinary field. The journal covers a wide range of topics, from fundamental research in physics, chemistry, and biology, including computational work and simulations, to the development of innovative devices and technologies for various industrial sectors such as information technology, medicine, manufacturing, high-performance materials, energy, and environmental technologies. It includes coverage of organic, inorganic, and hybrid materials.
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