Clustering of emission–dispersion dynamics in a state space defined by pollution sources and meteorological variables

IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Yuval , Yoav Levi , Pavel Khain , David M. Broday
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Abstract

The complex relationship between air pollution sources, the meteorological conditions governing their dispersion, and the resulting pollutant concentrations is an interesting scientific topic with significant implications for air resource management. A widely adopted approach to exploring these interactions is the interpretation of statistical models which simulate them. Dispersion conditions can vary markedly—from cold, calm nights with stable atmosphere to stormy periods characterised by intense turbulence and convection. Deeper insights can be obtained by interpreting statistical models trained on data subsets that correspond to specific emission–dispersion conditions. To achieve such distinct subsets, we present a robust and reproducible methodology for partitioning the multidimensional state space, defined by pollution sources and meteorological variables, into a large number of clusters at each monitoring location. Our methodology ensures a systematic and objective analysis across multiple stations. We analyse four years of hourly data, integrating high-resolution meteorological outputs from a numerical weather prediction model with traffic volume data used as proxies for emissions or precursors of NO, NO2, NOx, PM2.5, and O3 concentrations. These pollutants were observed at 85 air quality monitoring stations across Israel. The resulting clusters capture sub-daily temporal patterns that are indicative of distinct emission–dispersion scenarios in the region. We demonstrate that statistical models trained on these clustered subsets consistently outperform models trained on the full-period datasets. This highlights the value of our clustering approach in improving both predictive performance and scientific understanding of air pollution dispersion dynamics.

Abstract Image

由污染源和气象变量定义的状态空间中排放-扩散动力学的聚类
空气污染源、控制其扩散的气象条件和由此产生的污染物浓度之间的复杂关系是一个有趣的科学话题,对空气资源管理具有重要意义。探索这些相互作用的一种广泛采用的方法是解释模拟它们的统计模型。分散条件可以有明显的变化——从寒冷、平静的夜晚和稳定的大气,到以强烈湍流和对流为特征的暴风雨时期。通过解释在与特定排放扩散条件相对应的数据子集上训练的统计模型,可以获得更深入的见解。为了实现这些不同的子集,我们提出了一种健壮且可重复的方法,用于将由污染源和气象变量定义的多维状态空间划分为每个监测位置的大量集群。我们的方法确保在多个站点进行系统和客观的分析。我们分析了四年的每小时数据,将数值天气预报模型的高分辨率气象输出与交通量数据相结合,作为NO、NO2、NOx、PM2.5和O3浓度的排放或前驱物的代理。这些污染物是在以色列85个空气质量监测站观察到的。由此产生的集群捕获了亚日时间模式,这些模式表明了该地区不同的排放-扩散情景。我们证明了在这些聚类子集上训练的统计模型始终优于在全周期数据集上训练的模型。这突出了我们的聚类方法在提高预测性能和对空气污染扩散动力学的科学理解方面的价值。
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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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