Dual-Functional Evaporator: Synergistic Seawater Purification via Photothermal Evaporation and Microplastic Adsorption

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Wanli Peng, Jie Wang, Yilin Shi, Jie Wang and Zaisheng Cai*, 
{"title":"Dual-Functional Evaporator: Synergistic Seawater Purification via Photothermal Evaporation and Microplastic Adsorption","authors":"Wanli Peng,&nbsp;Jie Wang,&nbsp;Yilin Shi,&nbsp;Jie Wang and Zaisheng Cai*,&nbsp;","doi":"10.1021/acsami.5c10916","DOIUrl":null,"url":null,"abstract":"<p >Freshwater scarcity and microplastic (MP) pollution are two pressing challenges that urgently demand solutions. Integrating solar-driven interfacial evaporation with MP adsorption provides an effective approach for seawater purification. In this work, we fabricated a dual-functional synergistic solar evaporator. This system simultaneously achieves MP adsorption and seawater desalination, overcoming the single-functional water treatment objective of traditional evaporators to establish a composite water purification system. This work assembled PEI-coated viscose fibers, hydrophilic cotton fabric, and a PTFE photothermal layer through sewing techniques. The resulting evaporator features a hydrophobic top layer and a bottom layer that is capable of supplying water and adsorbing MPs. Under 1 kW m<sup>–2</sup> irradiation, the evaporator achieved an evaporation rate of 2.18 kg·m<sup>–2</sup>·h<sup>–1</sup> while demonstrating good long-term stability in saline water. Additionally, it exhibits 99.20% adsorption efficiency for low-concentration MPs in water. Notably, the condensate produced by the evaporator contains no MPs due to the double-layer structure separating the adsorption unit and the photothermal component. Therefore, the designed evaporator demonstrates promising potential not only to alleviate freshwater scarcity but also to effectively remove MPs from aquatic environments.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"17 30","pages":"43740–43749"},"PeriodicalIF":8.2000,"publicationDate":"2025-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsami.5c10916","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Freshwater scarcity and microplastic (MP) pollution are two pressing challenges that urgently demand solutions. Integrating solar-driven interfacial evaporation with MP adsorption provides an effective approach for seawater purification. In this work, we fabricated a dual-functional synergistic solar evaporator. This system simultaneously achieves MP adsorption and seawater desalination, overcoming the single-functional water treatment objective of traditional evaporators to establish a composite water purification system. This work assembled PEI-coated viscose fibers, hydrophilic cotton fabric, and a PTFE photothermal layer through sewing techniques. The resulting evaporator features a hydrophobic top layer and a bottom layer that is capable of supplying water and adsorbing MPs. Under 1 kW m–2 irradiation, the evaporator achieved an evaporation rate of 2.18 kg·m–2·h–1 while demonstrating good long-term stability in saline water. Additionally, it exhibits 99.20% adsorption efficiency for low-concentration MPs in water. Notably, the condensate produced by the evaporator contains no MPs due to the double-layer structure separating the adsorption unit and the photothermal component. Therefore, the designed evaporator demonstrates promising potential not only to alleviate freshwater scarcity but also to effectively remove MPs from aquatic environments.

Abstract Image

双功能蒸发器:通过光热蒸发和微塑料吸附协同净化海水。
淡水短缺和微塑料污染是两个迫切需要解决的挑战。将太阳能驱动的界面蒸发与MP吸附相结合,为海水净化提供了有效途径。在这项工作中,我们制作了一个双功能的协同太阳能蒸发器。该系统同时实现了MP吸附和海水淡化,克服了传统蒸发器功能单一的水处理目标,建立了复合水净化系统。这项工作通过缝纫技术组装了涂有pei的粘胶纤维,亲水性棉织物和聚四氟乙烯光热层。由此产生的蒸发器具有疏水的顶层和能够供水和吸附MPs的底层。在1 kW m-2辐照下,蒸发器的蒸发速率为2.18 kg·m-2·h-1,在盐水中具有良好的长期稳定性。对水中低浓度MPs的吸附效率为99.20%。值得注意的是,蒸发器产生的冷凝水不含MPs,因为吸附单元和光热组件是双层结构分开的。因此,所设计的蒸发器显示出良好的潜力,不仅可以缓解淡水短缺,还可以有效地从水生环境中去除MPs。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信