Quantitative and mechanistic study of the effect of river valley topography on urban scale pollution dispersion

IF 7.6 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Ying Wang , Yuxuan Hao , Yanyan Zhou , Jianxiong Liu , Yanfei Dong , Jiaxin Long , Wei Li
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Abstract

This study investigates the influence of complex terrain on air pollution dispersion during a valley-basin pollution episode in Lanzhou, northwestern China, using the WRF-CALPUFF modeling system and terrain-modified sensitivity experiments to quantify these topographic effects and reveal their underlying mechanisms. Results indicate that orographic features increase NO2 concentrations in urban areas by approximately 30 % on average, while channeling effects enhance ventilation and reduce pollutants in northwestern valleys. Analysis of atmospheric dynamics and thermodynamics reveals that thermally-induced local circulations combined with topographic stagnation create recirculation zones that effectively trap pollutants, as evidenced by recirculation factor analysis showing pronounced accumulation in these zones compared to well-ventilated areas. Valley heat deficit (VHD) demonstrates a strong correlation with NO2 levels (R = 0.77), where elevated VHD coincides spatially with recirculation zones and pollution hotspots. The study identifies a critical VHD threshold of 1.4 MJ/m2, beyond which pollution episodes occur due to suppressed vertical mixing from enhanced atmospheric stability and restricted horizontal transport from terrain-induced flow blockage. These findings highlight how the combined effects of thermal stabilization and flow obstruction work synergistically to sustain pollution accumulation in mountainous regions. The research establishes a comprehensive framework that elucidates the coupled dynamic-thermodynamic mechanisms through which terrain characteristics modulate pollution dispersion patterns, offering valuable insights into boundary layer processes and airflow dynamics during pollution events, with important implications for understanding urban air quality deterioration in complex terrain environments.

Abstract Image

Abstract Image

流域地形对城市尺度污染扩散影响的定量与机理研究
本研究利用WRF-CALPUFF模拟系统和地形修正敏感性实验,研究了复杂地形对兰州流域污染事件中空气污染扩散的影响,并揭示了其潜在机制。结果表明,地形特征使城市NO2浓度平均增加约30%,而沟道效应增强了西北山谷的通风,减少了污染物。大气动力学和热力学分析表明,热诱导的局部环流与地形停滞相结合,形成了有效捕获污染物的再循环区,再循环因子分析表明,与通风良好的地区相比,这些区域的累积明显。谷热亏缺(VHD)与NO2水平呈较强的相关性(R=0.77),其中谷热亏缺的升高在空间上与再循环区和污染热点重合。该研究确定了1.4 MJ/m2的临界VHD阈值,超过该阈值后,由于大气稳定性增强抑制了垂直混合,地形引起的气流阻塞限制了水平输送,污染事件就会发生。这些发现强调了热稳定和流动阻碍如何协同作用,以维持山区的污染积累。该研究建立了一个全面的框架,阐明了地形特征调节污染扩散模式的动力-热力学耦合机制,为污染事件中边界层过程和气流动力学提供了有价值的见解,对理解复杂地形环境下城市空气质量恶化具有重要意义。
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来源期刊
Environmental Pollution
Environmental Pollution 环境科学-环境科学
CiteScore
16.00
自引率
6.70%
发文量
2082
审稿时长
2.9 months
期刊介绍: Environmental Pollution is an international peer-reviewed journal that publishes high-quality research papers and review articles covering all aspects of environmental pollution and its impacts on ecosystems and human health. Subject areas include, but are not limited to: • Sources and occurrences of pollutants that are clearly defined and measured in environmental compartments, food and food-related items, and human bodies; • Interlinks between contaminant exposure and biological, ecological, and human health effects, including those of climate change; • Contaminants of emerging concerns (including but not limited to antibiotic resistant microorganisms or genes, microplastics/nanoplastics, electronic wastes, light, and noise) and/or their biological, ecological, or human health effects; • Laboratory and field studies on the remediation/mitigation of environmental pollution via new techniques and with clear links to biological, ecological, or human health effects; • Modeling of pollution processes, patterns, or trends that is of clear environmental and/or human health interest; • New techniques that measure and examine environmental occurrences, transport, behavior, and effects of pollutants within the environment or the laboratory, provided that they can be clearly used to address problems within regional or global environmental compartments.
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