Sustainable biomass-based filter for high-efficiency PM0.3 filtration

IF 14.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Qingxiang Wang, Zhaoxuan Niu, Wanli Cheng, Ming Yang, Jie Yan, Jiqing Lu, Haijiao Yu, Yiying Yue, Yen Wei, Dong Wang, Shichao Zhang, Bin Ding, Guangping Han
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Abstract

Biomass materials have been widely used in various industries to achieve a carbon-neutral and sustainable society. Here, we show a heterogeneous corn-based precursor strategy that transforms low-value agricultural waste into structural air filters composed of alternating microfibers (2.61 ± 1.11 µm) with grooved surface and nanofibers (0.29 ± 0.18 µm). Utilizing a green solute-solvent system of zein derived from corn and cellulose extracted from corn straw, the process ensures sustainability across raw material sources, fabrication, filtration, and end-of-life degradation. By tailoring relative humidity and incorporating cellulose, an incomplete nonsolvent-induced phase separation is triggered, leading to a corn-based dual-network filter with high filtration performance (>99.99% PM0.3 removal) and low pressure drop (45 Pa). The life cycle assessment demonstrates that the corn-based filter results in lower carbon emissions and environmental impacts than petroleum-based filters. This work provides a promising pathway toward the development of sustainable and disposable filtration materials.

Abstract Image

可持续生物质基过滤器,高效过滤PM0.3
生物质材料已广泛应用于各个行业,以实现碳中和和可持续发展的社会。在这里,我们展示了一种基于玉米的异质前体策略,该策略将低价值农业废弃物转化为由具有沟槽表面的微纤维(2.61±1.11µm)和纳米纤维(0.29±0.18µm)交替组成的结构空气过滤器。利用从玉米中提取的玉米蛋白和从玉米秸秆中提取的纤维素的绿色溶质-溶剂系统,该工艺确保了原材料来源、制造、过滤和寿命结束降解的可持续性。通过调整相对湿度并加入纤维素,可以触发非溶剂诱导的不完全相分离,从而产生具有高过滤性能(99.99% PM0.3去除率)和低压降(45 Pa)的玉米基双网过滤器。生命周期评价表明,玉米基过滤器比石油基过滤器的碳排放和环境影响更低。这项工作为开发可持续和一次性过滤材料提供了一条有希望的途径。
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来源期刊
Nature Communications
Nature Communications Biological Science Disciplines-
CiteScore
24.90
自引率
2.40%
发文量
6928
审稿时长
3.7 months
期刊介绍: Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.
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