{"title":"Hyperuniform mixing of binary active spinners.","authors":"Rui Liu, Mingcheng Yang, Ke Chen","doi":"10.1039/d5sm00458f","DOIUrl":null,"url":null,"abstract":"<p><p>Spinner mixtures consisting of both clockwise and counterclockwise self-spinning particles are often expected to phase separate. However, we demonstrate that such a demixing is absent for dimer (or rod-like) spinners. These particles always mix, even in a globally-hyperuniform way, with the total structure factor <i>S</i>(<i>q</i> → 0) ∼ <i>q</i><sup><i>α</i></sup> (<i>α</i> > 0). This global hyperuniformity can be enhanced or weakened by changes in the driving torques or the particle density. The corresponding microscopic mechanism is attributed to the competition between a dynamical heterocoordination effect and effective like-particle attractions. Critical scaling for the absorbing state transition of the system is also found to persist, with a significant shift in its critical point observed. The system can be further thermalized, by the driving torques or through thermostating, into an ideal solution with identical partial radial distribution functions, which denies the possibility of being multi-hyperuniform. A simply-extended coupled density-oscillator theory explains why the system cannot be multi-hyperuniform, but can have a global hyperuniformity with the scaling exponent <i>α</i> approaching 2. Such a hyperuniform mixing provides a way to regulate the topological boundary flows of this chiral system, and this mixing regulation is found to barely affect the bulk density fluctuations, or even preserve the localization of the flows and the bulk hyperuniformity.</p>","PeriodicalId":103,"journal":{"name":"Soft Matter","volume":" ","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Soft Matter","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1039/d5sm00458f","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Spinner mixtures consisting of both clockwise and counterclockwise self-spinning particles are often expected to phase separate. However, we demonstrate that such a demixing is absent for dimer (or rod-like) spinners. These particles always mix, even in a globally-hyperuniform way, with the total structure factor S(q → 0) ∼ qα (α > 0). This global hyperuniformity can be enhanced or weakened by changes in the driving torques or the particle density. The corresponding microscopic mechanism is attributed to the competition between a dynamical heterocoordination effect and effective like-particle attractions. Critical scaling for the absorbing state transition of the system is also found to persist, with a significant shift in its critical point observed. The system can be further thermalized, by the driving torques or through thermostating, into an ideal solution with identical partial radial distribution functions, which denies the possibility of being multi-hyperuniform. A simply-extended coupled density-oscillator theory explains why the system cannot be multi-hyperuniform, but can have a global hyperuniformity with the scaling exponent α approaching 2. Such a hyperuniform mixing provides a way to regulate the topological boundary flows of this chiral system, and this mixing regulation is found to barely affect the bulk density fluctuations, or even preserve the localization of the flows and the bulk hyperuniformity.
期刊介绍:
Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.