Hyperuniform mixing of binary active spinners.

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL
Soft Matter Pub Date : 2025-07-15 DOI:10.1039/d5sm00458f
Rui Liu, Mingcheng Yang, Ke Chen
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引用次数: 0

Abstract

Spinner mixtures consisting of both clockwise and counterclockwise self-spinning particles are often expected to phase separate. However, we demonstrate that such a demixing is absent for dimer (or rod-like) spinners. These particles always mix, even in a globally-hyperuniform way, with the total structure factor S(q → 0) ∼ qα (α > 0). This global hyperuniformity can be enhanced or weakened by changes in the driving torques or the particle density. The corresponding microscopic mechanism is attributed to the competition between a dynamical heterocoordination effect and effective like-particle attractions. Critical scaling for the absorbing state transition of the system is also found to persist, with a significant shift in its critical point observed. The system can be further thermalized, by the driving torques or through thermostating, into an ideal solution with identical partial radial distribution functions, which denies the possibility of being multi-hyperuniform. A simply-extended coupled density-oscillator theory explains why the system cannot be multi-hyperuniform, but can have a global hyperuniformity with the scaling exponent α approaching 2. Such a hyperuniform mixing provides a way to regulate the topological boundary flows of this chiral system, and this mixing regulation is found to barely affect the bulk density fluctuations, or even preserve the localization of the flows and the bulk hyperuniformity.

二元主动旋丝的超均匀混合。
由顺时针和逆时针自旋粒子组成的旋转器混合物通常被认为是相分离的。然而,我们证明了二聚体(或棒状)纺丝体不存在这种分离。这些粒子总是以总结构因子S(q→0)~ qα (α >)混合,甚至以全局超均匀的方式混合。这种全局超均匀性可以通过驱动转矩或粒子密度的变化而增强或减弱。相应的微观机制归因于动态异位效应和有效的类粒子引力之间的竞争。系统吸收态转变的临界尺度也被发现持续存在,观察到其临界点的显著变化。该系统可以通过驱动力矩或恒温器进一步热化成具有相同部分径向分布函数的理想解,从而否认了多重超均匀的可能性。一个简单扩展的耦合密度振荡器理论解释了为什么系统不能是多重超均匀的,但可以具有全局超均匀性,且标度指数α接近2。这种超均匀混合为调节该手性体系的拓扑边界流动提供了一种方法,并且发现这种混合调节几乎不影响体密度波动,甚至保持了流动的局域化和体的超均匀性。
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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.
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