Types of regional and localised new aerosol particle formation and growth processes: Atmospheric Banana Atlas

IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES
Imre Salma, Tamás Weidinger, János Rohonczy, Máté Vörösmarty
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引用次数: 0

Abstract

The structure and variability of atmospheric new particle formation and particle diameter growth (NPF&G) processes provide valuable insights into the underlying chemical, physical and meteorological mechanisms including atmospheric mixing and transport-related effects. Therefore, we systematically categorised and characterised the NPF&G events observed over 13 years in an urban environment. Six regional-scale banana plot types with narrow onset, broad onset, arch shape, double onset, tandem growth and nocturnal occurrence were identified. Additionally, two localised types were defined: one exhibiting multiple, but underdeveloped banana shapes, and another with diverse angulate structures, both being limited in time. The localised processes typically occurred on 7% of days, and produced high (up to 60 × 103 cm−3) ultrafine particle number concentrations. Regional and localised processes can also happen on the same day. Our findings highlight the need to extend current NPF&G identification and classification frameworks by incorporating an additional step to distinguish localised events from regional processes.

Abstract Image

区域和局部新气溶胶粒子形成和生长过程的类型:大气香蕉地图集
大气新颗粒形成和颗粒直径增长(npf&g)过程的结构和变异为了解潜在的化学、物理和气象机制(包括大气混合和运输相关效应)提供了有价值的见解。因此,我们系统地对13年来在城市环境中观测到的npf&g事件进行了分类和表征。鉴定出6种区域尺度香蕉样地类型,分别为窄型、宽型、拱形、双型、串联生长和夜间发生。此外,还定义了两种局部类型:一种表现出多种但不发达的香蕉形状,另一种具有多种角度结构,两者在时间上都是有限的。局部过程通常发生在7%的天,并产生高(高达60 × 103 cm−3)的超细颗粒数量浓度。区域性和地方性的流程也可以在同一天进行。我们的研究结果强调,需要通过纳入一个额外的步骤来区分局部事件和区域过程,从而扩展当前的npf&g识别和分类框架。
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来源期刊
npj Climate and Atmospheric Science
npj Climate and Atmospheric Science Earth and Planetary Sciences-Atmospheric Science
CiteScore
8.80
自引率
3.30%
发文量
87
审稿时长
21 weeks
期刊介绍: npj Climate and Atmospheric Science is an open-access journal encompassing the relevant physical, chemical, and biological aspects of atmospheric and climate science. The journal places particular emphasis on regional studies that unveil new insights into specific localities, including examinations of local atmospheric composition, such as aerosols. The range of topics covered by the journal includes climate dynamics, climate variability, weather and climate prediction, climate change, ocean dynamics, weather extremes, air pollution, atmospheric chemistry (including aerosols), the hydrological cycle, and atmosphere–ocean and atmosphere–land interactions. The journal welcomes studies employing a diverse array of methods, including numerical and statistical modeling, the development and application of in situ observational techniques, remote sensing, and the development or evaluation of new reanalyses.
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