Diverse MOFs-derived carbon-based materials for advanced electrochemical energy applications

IF 23.8 Q1 CHEMISTRY, MULTIDISCIPLINARY

EnergyChem Pub Date : 2025-07-01 DOI:10.1016/j.enchem.2025.100163

Chun-Yan Yang , Jian-Ping Lang

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Abstract

Metal-organic frameworks (MOFs)-derived carbon-based materials have garnered significant attention in electrochemical energy storage and conversion owing to their tunable porous structures, compositional flexibility, and structural diversity. This review categorizes typical synthetic strategies for MOFs-derived carbon-based materials, while highlights their cutting-edge applications in two key domains in recent years: (1) electrocatalytic reactions, mainly encompassing hydrogen evolution reaction, oxygen evolution reaction, oxygen reduction reaction, and nitrogen reduction reaction; and (2) electrochemical energy storage systems, with a focus on lithium-ion batteries and sodium-ion batteries. Particular emphasis is placed on elucidating the critical structure-property relationships governing the performance of these functional materials. Finally, we present a forward-looking perspective addressing current challenges and future research directions, offering strategic insights for designing novel high-performance electrochemical materials through rational engineering of the architectures of MOFs-derived carbon-based materials.

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多种mofs衍生的碳基材料用于先进的电化学能源应用

金属有机骨架（MOFs）衍生的碳基材料由于其可调节的多孔结构、成分的灵活性和结构的多样性，在电化学能量存储和转换方面受到了广泛的关注。本文对mofs衍生碳基材料的典型合成策略进行了分类，重点介绍了近年来mofs衍生碳基材料在两个关键领域的前沿应用：(1)电催化反应，主要包括析氢反应、析氧反应、氧还原反应和氮还原反应；(2)电化学储能系统，重点是锂离子电池和钠离子电池。特别强调的是阐明控制这些功能材料性能的关键结构-性能关系。最后，我们提出了前瞻性的观点，解决了当前的挑战和未来的研究方向，为通过合理的mofs衍生碳基材料结构工程设计新型高性能电化学材料提供了战略见解。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

EnergyChem Multiple-

CiteScore

40.80

自引率

2.80%

发文量

审稿时长

40 days

期刊介绍： EnergyChem, a reputable journal, focuses on publishing high-quality research and review articles within the realm of chemistry, chemical engineering, and materials science with a specific emphasis on energy applications. The priority areas covered by the journal include:Solar energy,Energy harvesting devices,Fuel cells,Hydrogen energy,Bioenergy and biofuels,Batteries,Supercapacitors,Electrocatalysis and photocatalysis,Energy storage and energy conversion,Carbon capture and storage