Correlation between the dome-shaped superconducting phase diagram, charge order, and normal-state electronic properties in LaRu3Si2.

IF 14.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
KeYuan Ma, Igor Plokhikh, Jennifer N Graham, Charles Mielke Iii, Vahid Sazgari, Hiroto Nakamura, Shams Sohel Islam, Soohyeon Shin, Petr Král, Orion Gerguri, Hubertus Luetkens, Fabian O von Rohr, Jiaxin Yin, Ekaterina Pomjakushina, Claudia Felser, Satoru Nakatsuji, Björn Wehinger, Dariusz J Gawryluk, Sergey Medvedev, Zurab Guguchia
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Abstract

The interplay between superconductivity and charge or spin order is a key focus in condensed matter physics, with kagome lattice systems providing unique insights. The kagome superconductor LaRu3Si2 (Tc ≃ 6.5 K) features a characteristic kagome band structure and a hierarchy of charge order transitions at Tco,I ≃ 400 K and Tco,II ≃ 80 K, along with an additional transition at T* ≃ 35 K associated with electronic and magnetic responses. Using magnetotransport under pressure up to 40 GPa, we find Tc peaks at 9 K (2 GPa)-the highest among kagome superconductors-remains nearly constant up to 12 GPa, and then decreases to 2 K at 40 GPa, forming a dome-shaped phase diagram. Similarly, both the resistivity anomaly at T* and the magnetoresistance exhibit a dome-shaped pressure dependence. Moreover, above 12 GPa, X-ray diffraction reveals that the charge order evolves from long-range to short-range, coinciding with the suppression of Tc. These observations indicate that superconductivity in LaRu3Si2 is closely linked to the charge-ordered state and the electronic responses at Tco,II and T*.

LaRu3Si2中圆顶超导相图、电荷序与正态电子性质的关系。
超导性与电荷或自旋顺序之间的相互作用是凝聚态物理的一个关键焦点,kagome晶格系统提供了独特的见解。kagome超导体LaRu3Si2 (Tc≃6.5 K)具有kagome带结构特征,在Tco,I≃400 K和Tco,II≃80 K处存在电荷阶跃,在T*≃35 K处存在与电子和磁响应相关的电荷阶跃。在高达40 GPa的压力下使用磁输运,我们发现kagome超导体中最高的9 K (2 GPa)的Tc峰值在12 GPa时几乎保持不变,然后在40 GPa时下降到2 K,形成圆顶状相图。同样,T*处的电阻率异常和磁阻都表现出圆顶状的压力依赖关系。在12 GPa以上,x射线衍射显示电荷顺序由远程向近程演变,与Tc的抑制一致。这些观察结果表明,LaRu3Si2中的超导性与电荷有序态和Tco,II和T*处的电子响应密切相关。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Nature Communications
Nature Communications Biological Science Disciplines-
CiteScore
24.90
自引率
2.40%
发文量
6928
审稿时长
3.7 months
期刊介绍: Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.
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