KeYuan Ma, Igor Plokhikh, Jennifer N Graham, Charles Mielke Iii, Vahid Sazgari, Hiroto Nakamura, Shams Sohel Islam, Soohyeon Shin, Petr Král, Orion Gerguri, Hubertus Luetkens, Fabian O von Rohr, Jiaxin Yin, Ekaterina Pomjakushina, Claudia Felser, Satoru Nakatsuji, Björn Wehinger, Dariusz J Gawryluk, Sergey Medvedev, Zurab Guguchia
{"title":"Correlation between the dome-shaped superconducting phase diagram, charge order, and normal-state electronic properties in LaRu<sub>3</sub>Si<sub>2</sub>.","authors":"KeYuan Ma, Igor Plokhikh, Jennifer N Graham, Charles Mielke Iii, Vahid Sazgari, Hiroto Nakamura, Shams Sohel Islam, Soohyeon Shin, Petr Král, Orion Gerguri, Hubertus Luetkens, Fabian O von Rohr, Jiaxin Yin, Ekaterina Pomjakushina, Claudia Felser, Satoru Nakatsuji, Björn Wehinger, Dariusz J Gawryluk, Sergey Medvedev, Zurab Guguchia","doi":"10.1038/s41467-025-61383-z","DOIUrl":null,"url":null,"abstract":"<p><p>The interplay between superconductivity and charge or spin order is a key focus in condensed matter physics, with kagome lattice systems providing unique insights. The kagome superconductor LaRu<sub>3</sub>Si<sub>2</sub> (T<sub>c</sub> ≃ 6.5 K) features a characteristic kagome band structure and a hierarchy of charge order transitions at T<sub>co,I</sub> ≃ 400 K and T<sub>co,II</sub> ≃ 80 K, along with an additional transition at T* ≃ 35 K associated with electronic and magnetic responses. Using magnetotransport under pressure up to 40 GPa, we find T<sub>c</sub> peaks at 9 K (2 GPa)-the highest among kagome superconductors-remains nearly constant up to 12 GPa, and then decreases to 2 K at 40 GPa, forming a dome-shaped phase diagram. Similarly, both the resistivity anomaly at T* and the magnetoresistance exhibit a dome-shaped pressure dependence. Moreover, above 12 GPa, X-ray diffraction reveals that the charge order evolves from long-range to short-range, coinciding with the suppression of T<sub>c</sub>. These observations indicate that superconductivity in LaRu<sub>3</sub>Si<sub>2</sub> is closely linked to the charge-ordered state and the electronic responses at T<sub>co,II</sub> and T*.</p>","PeriodicalId":19066,"journal":{"name":"Nature Communications","volume":"16 1","pages":"6149"},"PeriodicalIF":14.7000,"publicationDate":"2025-07-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature Communications","FirstCategoryId":"103","ListUrlMain":"https://doi.org/10.1038/s41467-025-61383-z","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
引用次数: 0
Abstract
The interplay between superconductivity and charge or spin order is a key focus in condensed matter physics, with kagome lattice systems providing unique insights. The kagome superconductor LaRu3Si2 (Tc ≃ 6.5 K) features a characteristic kagome band structure and a hierarchy of charge order transitions at Tco,I ≃ 400 K and Tco,II ≃ 80 K, along with an additional transition at T* ≃ 35 K associated with electronic and magnetic responses. Using magnetotransport under pressure up to 40 GPa, we find Tc peaks at 9 K (2 GPa)-the highest among kagome superconductors-remains nearly constant up to 12 GPa, and then decreases to 2 K at 40 GPa, forming a dome-shaped phase diagram. Similarly, both the resistivity anomaly at T* and the magnetoresistance exhibit a dome-shaped pressure dependence. Moreover, above 12 GPa, X-ray diffraction reveals that the charge order evolves from long-range to short-range, coinciding with the suppression of Tc. These observations indicate that superconductivity in LaRu3Si2 is closely linked to the charge-ordered state and the electronic responses at Tco,II and T*.
期刊介绍:
Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.