Energy and Clean Air Policies Will Overcome the Adverse Effect of Climate Change and Reduce China's Ozone Pollution in the Future: The Insight From a New Two-Stage Model

IF 3.4 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES
Yutong Wang, Yu Zhao
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引用次数: 0

Abstract

Near-surface ozone pollution is one of the biggest challenges for Chinese air quality improvement, whereas its future spatiotemporal evolution and driving factors have not been fully investigated. Here, we developed a two-stage model combining a machine learning technique (XGBoost) and a chemical transport model (WRF-CMAQ) to assess the ozone change till 2060 in China under three scenarios with various trajectories of climate change, energy transition, and pollution controls. The new model effectively corrected overestimation and underestimation of ozone levels by WRF-CMAQ and global climate models, respectively. Anthropogenic efforts will overcome the adverse effect of climate and reduce future ozone concentration especially in eastern China and warm season with greater ozone pollution. From a long-term perspective, energy structure transition was estimated to play a more important role than end-of-pipe emission controls with a former to latter ratio of ozone reduction during 2017–2060 at 2.7. With observational information incorporated, our model was demonstrated to better capture the ozone response to precursor emission change than WRF-CMAQ and corrected the underestimation of ozone reduction for developed urban areas.

能源和清洁空气政策将在未来克服气候变化的不利影响并减少中国的臭氧污染:一个新的两阶段模型的见解
近地表臭氧污染是中国空气质量改善面临的最大挑战之一,但其未来时空演变及其驱动因素尚未得到充分研究。在此,我们开发了一个结合机器学习技术(XGBoost)和化学输运模型(WRF-CMAQ)的两阶段模型,以评估在气候变化、能源转型和污染控制的不同轨迹下,中国到2060年的臭氧变化。新模式有效地修正了WRF-CMAQ模式和全球气候模式对臭氧水平的高估和低估。人为活动将克服气候的不利影响,降低未来的臭氧浓度,特别是在臭氧污染较严重的华东和暖季。从长期来看,能源结构转型比末端排放控制发挥更重要的作用,2017-2060年臭氧减排的前者与后者之比为2.7。与WRF-CMAQ模型相比,该模型能够更好地捕捉臭氧对前体排放变化的响应,并修正了对发达城市地区臭氧减少的低估。
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来源期刊
Journal of Geophysical Research: Atmospheres
Journal of Geophysical Research: Atmospheres Earth and Planetary Sciences-Geophysics
CiteScore
7.30
自引率
11.40%
发文量
684
期刊介绍: JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.
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