Zongyun Shao , Liqin Fu , Zhiqian Wang , Min Huang , Kun Jia , Nizao Kong , Ruibang Xie , Chiyu Wen , Kaiwen Hou , Fei Han
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引用次数: 0
Abstract
Thermal management issues in electronics force thermal interface materials (TIMs) possessing both high thermal conductivity and excellent resilience, but simultaneously achieving these properties in TIMs remains challenging. In this paper, TIMs with both high thermal conductivity and mechanical properties are prepared by vertically aligning long mesophase pitch-based carbon fibers (CFs) in a simple lay-up method. The vertically aligned long CFs can not only minimize the thermal conductivity channels and maximize the number of the channels, but also provide structural support for the soft silicone rubber (SR) matrix, thus enabling TIMs to obtain both excellent thermal conductivity and mechanical properties. As a result, the prepared composite with a CFs content of 70 wt% possesses through-plane thermal conductivity up to 28.4 W m−1 K−1. In addition, the composite exhibits impressive mechanical properties, including a low Shore 00 hardness of 61, a high compressibility of 63.8 %, and superior rebound rate of 82 % under 45 psi pressure. With this high filler ratio, the stunning results highlight the potential of the carbon fiber arrays-filled composite for the advanced thermal management applications, which provides a reference scheme for further fabrication of high-performance resilient TIMs.
期刊介绍:
Composites Communications (Compos. Commun.) is a peer-reviewed journal publishing short communications and letters on the latest advances in composites science and technology. With a rapid review and publication process, its goal is to disseminate new knowledge promptly within the composites community. The journal welcomes manuscripts presenting creative concepts and new findings in design, state-of-the-art approaches in processing, synthesis, characterization, and mechanics modeling. In addition to traditional fiber-/particulate-reinforced engineering composites, it encourages submissions on composites with exceptional physical, mechanical, and fracture properties, as well as those with unique functions and significant application potential. This includes biomimetic and bio-inspired composites for biomedical applications, functional nano-composites for thermal management and energy applications, and composites designed for extreme service environments.