Diagnostic-free onboard battery health assessment

IF 38.6 1区 材料科学 Q1 CHEMISTRY, PHYSICAL
Joule Pub Date : 2025-06-30 DOI:10.1016/j.joule.2025.102010
Yunhong Che, Vivek N. Lam, Jinwook Rhyu, Joachim Schaeffer, Minsu Kim, Martin Z. Bazant, William C. Chueh, Richard D. Braatz
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引用次数: 0

Abstract

Diverse usage patterns induce complex and variable aging behaviors in lithium-ion batteries, complicating accurate health diagnosis and prognosis. In this work, we leverage portions of operational measurements from charging or dynamic discharging in combination with an interpretable machine learning model to enable rapid, onboard battery health diagnostics and prognostics without offline diagnostic testing and access to historical data. We integrate mechanistic constraints derived from differential voltage analysis within an encoder-decoder to extract electrode health states in a physically interpretable latent space, which enables improved reconstruction of the degradation path with onboard aging mechanisms tracking. The diagnosis model can be flexibly applied across diverse applications with slight fine-tuning. We demonstrate the model’s versatility by applying it to three battery-cycling datasets consisting of 422 cells under different operating conditions, with a mean absolute error of less than 2% for health diagnosis under varying conditions, highlighting the utility of an interpretable, diagnostic-free model.

Abstract Image

无诊断的机载电池健康评估
不同的使用模式导致锂离子电池复杂多变的老化行为,使准确的健康诊断和预后复杂化。在这项工作中,我们利用充电或动态放电的部分操作测量数据与可解释的机器学习模型相结合,实现快速的车载电池健康诊断和预测,而无需离线诊断测试和访问历史数据。我们在编码器-解码器中集成了来自差分电压分析的机械约束,以在物理可解释的潜在空间中提取电极健康状态,从而能够通过板载老化机制跟踪改进退化路径的重建。该诊断模型可以灵活地应用于不同的应用,只需稍作微调。我们通过将该模型应用于不同操作条件下由422个电池组成的三个电池循环数据集,证明了该模型的多功能性,在不同条件下进行健康诊断的平均绝对误差小于2%,突出了可解释的无诊断模型的实用性。
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来源期刊
Joule
Joule Energy-General Energy
CiteScore
53.10
自引率
2.00%
发文量
198
期刊介绍: Joule is a sister journal to Cell that focuses on research, analysis, and ideas related to sustainable energy. It aims to address the global challenge of the need for more sustainable energy solutions. Joule is a forward-looking journal that bridges disciplines and scales of energy research. It connects researchers and analysts working on scientific, technical, economic, policy, and social challenges related to sustainable energy. The journal covers a wide range of energy research, from fundamental laboratory studies on energy conversion and storage to global-level analysis. Joule aims to highlight and amplify the implications, challenges, and opportunities of novel energy research for different groups in the field.
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