A motile rod in an active nematic medium: caging, orientational trapping, and anomalous diffusion.

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL
Soft Matter Pub Date : 2025-06-27 DOI:10.1039/d5sm00573f
Abhishek Sharma, Harsh Soni
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Abstract

We study the dynamical and statistical properties of a motile polar rod embedded in a vibrated granular medium composed of fore-aft symmetric rods using particle-based numerical simulations. Our study reveals phase-dependent memory effects and transport behaviors of the polar rod governed by the structural phase of the medium. In the isotropic phase, the rod behaves as an active Brownian particle, experiencing a noisy environment with increasing medium concentration that leads to short-lived directional memory, resulting in enhanced rotational diffusion and reduced translational diffusivity. In the nematic phase-determined by the medium's concentration and the polar rod's intrinsic rotational noise-the rod exhibits two distinct states: a rotationally trapped state, in which its orientation is locked along the nematic director, and a rotationally free state, in which it explores all orientations despite a tendency to align with the director. At high concentrations, the medium forms periodic layers in which the rods are slightly tilted in opposite directions across adjacent layers relative to the nematic director, as reported by Sharma et al. [Soft Matter, 2024, 20, 6608-6617]. In this regime, the motile rod is effectively caged in the direction perpendicular to the nematic alignment. We further study the diffusive behavior of the polar rod in both states, demonstrating that the phase of the medium strongly influences its diffusion dynamics and the MSD exponent values, revealing a wide range of behavior from normal to superdiffusive dynamics.

活动向列介质中的活动棒:笼化、定向捕获和异常扩散。
我们利用基于粒子的数值模拟研究了嵌入在由前后对称杆组成的振动颗粒介质中的运动极棒的动力学和统计特性。我们的研究揭示了相依赖的记忆效应和极性棒的输运行为受介质结构相的支配。在各向同性阶段,棒表现为活跃的布朗粒子,经历介质浓度增加的嘈杂环境,导致短暂的定向记忆,从而增强旋转扩散和平移扩散率降低。在向列相(由介质浓度和极棒固有的旋转噪声决定)中,极棒表现出两种不同的状态:一种是旋转捕获状态,其方向沿着向列方向锁定;另一种是旋转自由状态,在这种状态下,它探索所有方向,尽管倾向于与方向对齐。根据Sharma等人的报道,高浓度的介质会形成周期性层,在这些层中,相对于向列导向,棒在相邻层中略微向相反方向倾斜。[软物质,2024,20,6608-6617]。在这种情况下,运动杆在垂直于向列对齐的方向上被有效地笼住。我们进一步研究了极性棒在两种状态下的扩散行为,表明介质的相位强烈影响其扩散动力学和MSD指数值,揭示了从正常到超扩散动力学的广泛行为。
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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.
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