Dianmeng Dong, Min Peng, Tao Zhang, Shichao Zhang, Xiaotong Ma, Yuanjun Tang, Yilin Cao, Qingyi Zhang, Fan Zhang, Yang Zhang, Zhenping Wu
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引用次数: 0
Abstract
Solar-blind photodetectors operating in the deep ultraviolet (DUV) spectrum are critical for applications. However, the severe attenuation of DUV signals in the atmosphere demands photodetectors with ultralow noise and high sensitivity to resolve weak optical signals. Here, we report a breakthrough in β-Ga2O3-based n-Barrier-n (nBn) unipolar heterostructure photodetectors that synergistically address these challenges. By employing a β-Ga2O3/LaAlO3/Nb:SrTiO3 heterojunction fabricated via laser molecular beam epitaxy, we engineer a large conduction band offset and near-zero valence band offset, creating a unipolar electron transport channel that suppresses dark current to subpicoampere levels (<1 pA). The device exhibits exceptional performance metrics: a responsivity of 853.6 A/W, an external quantum efficiency of 4.2 × 105%, and a record-low noise-equivalent power (NEP) of 0.7 ± 0.1 fW/Hz1/2─surpassing state-of-the-art DUV detectors. These advancements are attributed to the high dielectric constant (∼24) and lattice compatibility of LaAlO3 with Nb:SrTiO3, which minimize interfacial defects and enhance carrier confinement. This work not only establishes a new paradigm for Ga2O3-based optoelectronics but also provides a universal design strategy for high-sensitivity, low-noise photodetectors in photon-starved environments, with transformative potential for deep-space communication and ultraviolet astronomy.
期刊介绍:
Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.