Recent Advances in Heterogeneous Frustrated Lewis Pair: Synthesis, Characterization, and Catalysi.

IF 27.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jiasi Li,Shik Chi Edman Tsang,Guangchao Li
{"title":"Recent Advances in Heterogeneous Frustrated Lewis Pair: Synthesis, Characterization, and Catalysi.","authors":"Jiasi Li,Shik Chi Edman Tsang,Guangchao Li","doi":"10.1002/adma.202502101","DOIUrl":null,"url":null,"abstract":"Frustrated Lewis pair (FLP) in heterogeneous chemistry have garnered tremendous attention in recent years owing to their diverse structural designs and outstanding activation ability for small molecules. The ability to tailor the structure of FLP enables precise control over their reactivity and selectivity, paving the way for the creation of catalysts for specific reactions. This review offers an in-depth examination of the design, characterization, and application of FLP within heterogeneous systems over the past few years. The current challenges in developing solid FLP catalysts are discussed. Furthermore, future potential advancements are explored, considering how emerging technologies and innovative approaches could enhance the design, advance characterization, and application of FLP in heterogeneous chemistry. Through this detailed overview, it is aimed to provide valuable insights into the evolving landscape of FLP research and its implications for the future applications in catalysis.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"45 1","pages":"e2502101"},"PeriodicalIF":27.4000,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adma.202502101","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Frustrated Lewis pair (FLP) in heterogeneous chemistry have garnered tremendous attention in recent years owing to their diverse structural designs and outstanding activation ability for small molecules. The ability to tailor the structure of FLP enables precise control over their reactivity and selectivity, paving the way for the creation of catalysts for specific reactions. This review offers an in-depth examination of the design, characterization, and application of FLP within heterogeneous systems over the past few years. The current challenges in developing solid FLP catalysts are discussed. Furthermore, future potential advancements are explored, considering how emerging technologies and innovative approaches could enhance the design, advance characterization, and application of FLP in heterogeneous chemistry. Through this detailed overview, it is aimed to provide valuable insights into the evolving landscape of FLP research and its implications for the future applications in catalysis.
非均相挫折路易斯对的合成、表征及催化研究进展。
受挫刘易斯对(FLP)由于其多样的结构设计和对小分子突出的活化能力,近年来在非均相化学中引起了广泛的关注。定制FLP结构的能力可以精确控制其反应性和选择性,为创造特定反应的催化剂铺平了道路。这篇综述对过去几年异质系统中FLP的设计、表征和应用进行了深入的研究。讨论了目前发展固体FLP催化剂面临的挑战。此外,还探讨了未来的潜在进展,考虑到新兴技术和创新方法如何增强FLP在多相化学中的设计,推进表征和应用。通过这一详细的概述,旨在为FLP研究的发展前景及其对未来催化应用的影响提供有价值的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Advanced Materials
Advanced Materials 工程技术-材料科学:综合
CiteScore
43.00
自引率
4.10%
发文量
2182
审稿时长
2 months
期刊介绍: Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信