Optimisation of electronic nose performance with multi-attention and domain adaptation for fire forensics

IF 2.6 3区 化学 Q2 CHEMISTRY, ANALYTICAL
Tian-Shu Song, Hui-Rang Hou and Qing-Hao Meng
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Abstract

The identification of ignitable liquids at fire scenes is a crucial component of forensic investigations. However, conventional analytical methods such as gas chromatography-mass spectrometry, often require costly equipment, specialised expertise, and extended analysis times, which limits their effectiveness for rapid on-site detection. As such, electronic nose (e-nose) technology presents a cost-effective and portable alternative. Nevertheless, inconsistencies in sensor responses across different platforms pose challenges to model transferability which requires independent data collection and model training for each device. This study introduces a multiple attention adversarial transfer learning (MAATL) network aimed at addressing cross-platform variability in ignitable liquid detection using e-noses. The MAATL framework incorporates a multiple attention mechanism to optimise sensor signals, a multi-scale one-dimensional convolutional network for feature extraction, and adversarial learning techniques to enhance domain adaptation. Experimental validation involved five e-nose platforms and four classes of ignitable liquids, namely gasoline, diesel, alcohol, and diluent. The results demonstrated an average classification accuracy of 87% with peak accuracy reaching as high as 97.3%. Furthermore, the Fréchet inception distance (FID) metric indicated significant distribution differences between e-nose platforms, with values ranging from 12.8 to 35.6. Overall, these findings suggest that the proposed method enhances the reliability and scalability of e-nose-based ignitable liquid detection, thereby contributing to more efficient forensic investigations and expanding potential applications in chemical sensing.

Abstract Image

基于多关注和领域适应的火灾取证电子鼻性能优化。
火灾现场可燃液体的鉴定是法医调查的重要组成部分。然而,传统的分析方法,如气相色谱-质谱法,通常需要昂贵的设备、专业知识和延长的分析时间,这限制了它们快速现场检测的有效性。因此,电子鼻技术提供了一种具有成本效益和便携性的替代方案。然而,不同平台之间传感器响应的不一致性对模型可移植性提出了挑战,这需要对每个设备进行独立的数据收集和模型训练。本研究引入了一种多注意对抗迁移学习(MAATL)网络,旨在解决使用电子鼻检测可燃液体的跨平台可变性。MAATL框架结合了一个多注意机制来优化传感器信号,一个多尺度一维卷积网络用于特征提取,以及对抗学习技术来增强领域适应。实验验证涉及五个电子鼻平台和四类可燃液体,即汽油,柴油,酒精和稀释剂。结果表明,平均分类准确率为87%,峰值准确率高达97.3%。此外,电子鼻平台之间的fr起始距离(FID)分布差异显著,其值在12.8 ~ 35.6之间。总的来说,这些发现表明,所提出的方法提高了基于电子鼻的可燃液体检测的可靠性和可扩展性,从而有助于更有效的法医调查和扩大化学传感的潜在应用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Analytical Methods
Analytical Methods CHEMISTRY, ANALYTICAL-FOOD SCIENCE & TECHNOLOGY
CiteScore
5.10
自引率
3.20%
发文量
569
审稿时长
1.8 months
期刊介绍: Early applied demonstrations of new analytical methods with clear societal impact
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