Temperature-Responsive Polymer Grafted Carbon Nanotubes for Active Control of Mineral Scaling

IF 16 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Xiaoyin Tian, Yifan Zhu*, Xiaochuan Huang, Yifeng Liu, Guanhui Gao, Qing Ai, Michelle T. Chen, Xintong Weng, Yuren Feng, Boyu Zhang, Tianshu Zhai, Qiyi Fang, Jun Lou* and Qilin Li*, 
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引用次数: 0

Abstract

Scaling presents a major challenge in water treatment industries, reducing operational efficiency and shortening the service life of membranes and plumbing systems. Frequent membrane replacement imposes a substantial economic burden. Traditional scale removal methods, including physical cleaning and chemical treatments, often cause membrane damage, environmental hazards, and additional costs. To address these challenges, this study developed an antideposition, self-cleaning membrane structure for combating scaling in water treatment. The membrane features a poly(N-isopropylacrylamide) coating grafted onto carbon nanotube surfaces, providing dual functionalities: temperature responsiveness and high conductivity. These properties enable polymer motion and bubble generation on the membrane surface upon application of electrical current. The polymer movement effectively reduces deposition during operation, while the bubbles generated during water splitting reactions act as a natural cleaning mechanism. This approach offers a sustainable and efficient solution to scaling issues in water treatment systems.

Abstract Image

温度响应聚合物接枝碳纳米管对矿物结垢的主动控制
结垢是水处理行业面临的主要挑战,它降低了操作效率,缩短了膜和管道系统的使用寿命。频繁的膜更换带来了巨大的经济负担。传统的除垢方法,包括物理清洗和化学处理,通常会造成膜损伤、环境危害和额外的成本。为了解决这些挑战,本研究开发了一种抗沉积、自清洁的膜结构,用于对抗水处理中的结垢。该膜的特点是将聚(n -异丙基丙烯酰胺)涂层接枝到碳纳米管表面,具有双重功能:温度响应性和高导电性。这些特性使聚合物在施加电流时能在膜表面运动并产生气泡。聚合物的运动有效地减少了操作过程中的沉积,而在水分解反应中产生的气泡则是一种天然的清洁机制。这种方法为水处理系统中的结垢问题提供了可持续和有效的解决方案。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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