Alexander Wilzewski, Lukas J. Spieß, Malte Wehrheim, Shuying Chen, Steven A. King, Peter Micke, Melina Filzinger, Martin R. Steinel, Nils Huntemann, Erik Benkler, Piet O. Schmidt, Luca I. Huber, Jeremy Flannery, Roland Matt, Martin Stadler, Robin Oswald, Fabian Schmid, Daniel Kienzler, Jonathan Home, Diana P. L. Aude Craik, Menno Door, Sergey Eliseev, Pavel Filianin, Jost Herkenhoff, Kathrin Kromer, Klaus Blaum, Vladimir A. Yerokhin, Igor A. Valuev, Natalia S. Oreshkina, Chunhai Lyu, Sreya Banerjee, Christoph H. Keitel, Zoltán Harman, Julian C. Berengut, Anna Viatkina, Jan Gilles, Andrey Surzhykov, Michael K. Rosner, José R. Crespo López-Urrutia, Jan Richter, Agnese Mariotti, Elina Fuchs
{"title":"Nonlinear Calcium King Plot Constrains New Bosons and Nuclear Properties","authors":"Alexander Wilzewski, Lukas J. Spieß, Malte Wehrheim, Shuying Chen, Steven A. King, Peter Micke, Melina Filzinger, Martin R. Steinel, Nils Huntemann, Erik Benkler, Piet O. Schmidt, Luca I. Huber, Jeremy Flannery, Roland Matt, Martin Stadler, Robin Oswald, Fabian Schmid, Daniel Kienzler, Jonathan Home, Diana P. L. Aude Craik, Menno Door, Sergey Eliseev, Pavel Filianin, Jost Herkenhoff, Kathrin Kromer, Klaus Blaum, Vladimir A. Yerokhin, Igor A. Valuev, Natalia S. Oreshkina, Chunhai Lyu, Sreya Banerjee, Christoph H. Keitel, Zoltán Harman, Julian C. Berengut, Anna Viatkina, Jan Gilles, Andrey Surzhykov, Michael K. Rosner, José R. Crespo López-Urrutia, Jan Richter, Agnese Mariotti, Elina Fuchs","doi":"10.1103/physrevlett.134.233002","DOIUrl":null,"url":null,"abstract":"Nonlinearities in King plots (KP) of isotope shifts (IS) can reveal the existence of beyond-standard-model (BSM) interactions that couple electrons and neutrons. However, it is crucial to distinguish higher-order standard model (SM) effects from BSM physics. We measure the IS of the transitions P</a:mi></a:mrow>3</a:mn></a:mrow></a:mmultiscripts></a:mrow>0</a:mn></a:mrow></a:msub>→</a:mo>P</a:mi></a:mrow>3</a:mn></a:mrow></a:mmultiscripts></a:mrow>1</a:mn></a:mrow></a:msub></a:mrow></a:math> in <d:math xmlns:d=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><d:mrow><d:msup><d:mrow><d:mi>Ca</d:mi></d:mrow><d:mrow><d:mn>14</d:mn><d:mo>+</d:mo></d:mrow></d:msup></d:mrow></d:math> and <f:math xmlns:f=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><f:mrow><f:msub><f:mrow><f:mmultiscripts><f:mrow><f:mi>S</f:mi></f:mrow><f:mprescripts/><f:none/><f:mrow><f:mn>2</f:mn></f:mrow></f:mmultiscripts></f:mrow><f:mrow><f:mn>1</f:mn><f:mo>/</f:mo><f:mn>2</f:mn></f:mrow></f:msub><f:mo stretchy=\"false\">→</f:mo><f:mmultiscripts><f:mrow><f:msub><f:mrow><f:mi>D</f:mi></f:mrow><f:mrow><f:mn>5</f:mn><f:mo>/</f:mo><f:mn>2</f:mn></f:mrow></f:msub></f:mrow><f:mprescripts/><f:none/><f:mrow><f:mn>2</f:mn></f:mrow></f:mmultiscripts></f:mrow></f:math> in <i:math xmlns:i=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><i:msup><i:mi>Ca</i:mi><i:mo>+</i:mo></i:msup></i:math> with sub-Hz precision as well as the nuclear mass ratios with relative uncertainties below <k:math xmlns:k=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><k:mn>4</k:mn><k:mo>×</k:mo><k:msup><k:mn>10</k:mn><k:mrow><k:mo>−</k:mo><k:mn>11</k:mn></k:mrow></k:msup></k:math> for the five stable, even isotopes of calcium (<m:math xmlns:m=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><m:mrow><m:mmultiscripts><m:mrow><m:mi>Ca</m:mi></m:mrow><m:mprescripts/><m:none/><m:mrow><m:mn>40</m:mn><m:mo>,</m:mo><m:mn>42</m:mn><m:mo>,</m:mo><m:mn>44</m:mn><m:mo>,</m:mo><m:mn>46</m:mn><m:mo>,</m:mo><m:mn>48</m:mn></m:mrow></m:mmultiscripts></m:mrow></m:math>). Combined, these measurements yield a calcium KP nonlinearity with a significance of <o:math xmlns:o=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><o:mo>∼</o:mo><o:msup><o:mn>10</o:mn><o:mn>3</o:mn></o:msup><o:mi>σ</o:mi></o:math>. Precision calculations show that the nonlinearity cannot be fully accounted for by the expected largest higher-order SM effect, the second-order mass shift, and identify the little-studied nuclear polarization as the only remaining SM contribution that may be large enough to explain it. Despite the observed nonlinearity, we improve existing KP-based constraints on a hypothetical Yukawa interaction for most of the new boson masses between <q:math xmlns:q=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><q:mrow><q:mn>10</q:mn><q:mtext> </q:mtext><q:mtext> </q:mtext><q:mi>eV</q:mi><q:mo>/</q:mo><q:msup><q:mrow><q:mi mathvariant=\"normal\">c</q:mi></q:mrow><q:mrow><q:mn>2</q:mn></q:mrow></q:msup></q:mrow></q:math> and <t:math xmlns:t=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><t:mrow><t:msup><t:mrow><t:mn>10</t:mn></t:mrow><t:mrow><t:mn>7</t:mn></t:mrow></t:msup><t:mtext> </t:mtext><t:mtext> </t:mtext><t:mi>eV</t:mi><t:mo>/</t:mo><t:msup><t:mrow><t:mi mathvariant=\"normal\">c</t:mi></t:mrow><t:mrow><t:mn>2</t:mn></t:mrow></t:msup></t:mrow></t:math>. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20069,"journal":{"name":"Physical review letters","volume":"588 1","pages":""},"PeriodicalIF":9.0000,"publicationDate":"2025-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical review letters","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physrevlett.134.233002","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Nonlinearities in King plots (KP) of isotope shifts (IS) can reveal the existence of beyond-standard-model (BSM) interactions that couple electrons and neutrons. However, it is crucial to distinguish higher-order standard model (SM) effects from BSM physics. We measure the IS of the transitions P30→P31 in Ca14+ and S21/2→D5/22 in Ca+ with sub-Hz precision as well as the nuclear mass ratios with relative uncertainties below 4×10−11 for the five stable, even isotopes of calcium (Ca40,42,44,46,48). Combined, these measurements yield a calcium KP nonlinearity with a significance of ∼103σ. Precision calculations show that the nonlinearity cannot be fully accounted for by the expected largest higher-order SM effect, the second-order mass shift, and identify the little-studied nuclear polarization as the only remaining SM contribution that may be large enough to explain it. Despite the observed nonlinearity, we improve existing KP-based constraints on a hypothetical Yukawa interaction for most of the new boson masses between 10eV/c2 and 107eV/c2. Published by the American Physical Society2025
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