Perovskite as a Promising Candidate for Treating Typical Contaminants in Medical Wastewater: Synthesis, Progress, and Mechanism

IF 3.9 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Xiaoyu Sun, Shiyu Sun, Ting Wang*, Xin Huang, Na Wang, Lina Zhou and Hongxun Hao*, 
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Abstract

With the fast development of global medical and health undertakings, medical wastewater has increasingly posed a great threat to human survival and ecosystems. This type of wastewater might contain many components, such as drugs, radioactive substances, heavy metals, etc., making it difficult to meet discharge standards. What is more, although efforts have been made to treat these pollutants, the incomplete degradation of pollutants or secondary pollution during treatment would inevitably complicate the problem. The core limitations of existing technologies lie in their inability to simultaneously achieve high adsorption capacity and thorough mineralization of contaminants, poor removal efficiency for low concentration of pollutants, and weak recyclability of the materials. These issues result in high operational costs and persistent environmental risks. In order to treat medical wastewater, researchers have proposed many methods. As one of the most effective adsorbents and photocatalysts, perovskites offer numerous benefits, including convenient recovery, lower price, high metal site activity, and wide light response range. This report summarizes approaches used to synthesize and modify perovskite. We discuss the application and associated mechanisms involved in remediating medical effluents and removing contaminants. Meanwhile, there will also be a comparison and discussion about effectiveness, limitations, and benefits of each handling approach. In addition, prospects and possible orientations of the perovskite are proposed. Results presented in this review will help researchers in the area of perovskite-based materials to find new research ideas or methods that could be used to synthesize new materials for treating other complex water bodies, which is of great scientific significance and application value for promoting the development of green water treatment technology and realizing the goal of environmentally sustainable development.

Abstract Image

钙钛矿作为处理医疗废水中典型污染物的有前途的候选者:合成、进展和机理
随着全球医疗卫生事业的快速发展,医疗废水对人类生存和生态系统的威胁越来越大。这类废水可能含有许多成分,如药物、放射性物质、重金属等,难以达到排放标准。更重要的是,尽管已经做出了努力来处理这些污染物,但在处理过程中污染物的不完全降解或二次污染将不可避免地使问题复杂化。现有技术的核心局限在于不能同时实现对污染物的高吸附量和彻底矿化,对低浓度污染物的去除效率较差,材料的可回收性较弱。这些问题导致高运营成本和持续的环境风险。为了处理医疗废水,研究人员提出了许多方法。钙钛矿作为最有效的吸附剂和光催化剂之一,具有回收方便、价格低廉、金属位活性高、光响应范围广等优点。本文综述了钙钛矿的合成和改性方法。我们讨论了在医疗废水修复和去除污染物方面的应用和相关机制。同时,还将对每种处理方法的有效性、局限性和益处进行比较和讨论。并对钙钛矿的发展前景和可能的方向进行了展望。本文综述的结果将有助于钙钛矿基材料领域的研究人员找到新的研究思路或方法,可用于合成处理其他复杂水体的新材料,对于促进绿色水处理技术的发展,实现环境可持续发展的目标具有重要的科学意义和应用价值。
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来源期刊
Langmuir
Langmuir 化学-材料科学:综合
CiteScore
6.50
自引率
10.30%
发文量
1464
审稿时长
2.1 months
期刊介绍: Langmuir is an interdisciplinary journal publishing articles in the following subject categories: Colloids: surfactants and self-assembly, dispersions, emulsions, foams Interfaces: adsorption, reactions, films, forces Biological Interfaces: biocolloids, biomolecular and biomimetic materials Materials: nano- and mesostructured materials, polymers, gels, liquid crystals Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do? Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*. This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).
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