High-Performance Ga2O3 In-Memory DUV Photodetectors By Interface Charge Reservoir Design for Multifunctional Applications

IF 27.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Xiaohu Hou, Chen Li, Chen Chen, Shiyu Bai, Yan liu, Zhixin Peng, Xiaolong Zhao, Xuanze Zhou, Guangwei Xu, Nan Gao, Shibing Long
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Abstract

The development of high-performance detectors has played a key role in the innovation of modern optoelectronics. However, the implementation of high-performance detectors has been a huge challenge, especially the present detectors with only optoelectronic conversion functions cannot satisfy the growing demands of the multifunction required in single devices. Here, it is demonstrated a novel in-memory photodetector based on wide bandgap semiconductor Ga2O3 by integrating memory characteristics into the detector. Originating from the dynamic control of the channel carriers by the interface charge reservoir under illumination and electrical, the device exhibits extraordinary memory characteristics and photodetection performance. The ultrahigh-speed programming/erasing operations in the range of nanoseconds with an extinction ratio up to 109 is achieved. Moreover, the in-memory photodetectors achieve near-zero dark current, record high responsivity (6.7 × 107 A W−1), and sensitivity for UV light, making them the most sensitive UV photodetectors. Further, the potential of the device in weak-light imaging enhancement, light information storage, and light moving path recording in the passive mode is excavated for the first time. This work enables new device capabilities and opens new opportunities for the development of high-performance in-memory detectors.

Abstract Image

多功能界面电荷库设计的高性能Ga2O3内存DUV光电探测器
高性能探测器的发展对现代光电子学的创新起着关键作用。然而,高性能探测器的实现一直是一个巨大的挑战,特别是目前只有光电转换功能的探测器无法满足单一器件日益增长的多功能需求。在这里,我们展示了一种基于宽禁带半导体Ga2O3的新型内存光电探测器,通过将存储特性集成到探测器中。该器件源于界面电荷库在光照和电作用下对通道载流子的动态控制,具有非凡的记忆特性和光探测性能。实现了纳秒范围内的超高速编程/擦除操作,消光比高达109。此外,存储器光电探测器实现了接近零的暗电流,记录了高响应率(6.7 × 107 A W−1)和对紫外光的灵敏度,使其成为最灵敏的紫外光探测器。此外,首次挖掘了该器件在弱光成像增强、光信息存储和无源模式下光移动路径记录方面的潜力。这项工作实现了新的设备功能,并为高性能内存检测器的开发开辟了新的机会。
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来源期刊
Advanced Materials
Advanced Materials 工程技术-材料科学:综合
CiteScore
43.00
自引率
4.10%
发文量
2182
审稿时长
2 months
期刊介绍: Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.
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