Dynamics and rupture of doped motility induced phase separation†

IF 2.8 3区 化学 Q3 CHEMISTRY, PHYSICAL
Soft Matter Pub Date : 2025-05-16 DOI:10.1039/D5SM00134J
Rodrigo Fernández-Quevedo García, Enrique Chacón, Pedro Tarazona and Chantal Valeriani
{"title":"Dynamics and rupture of doped motility induced phase separation†","authors":"Rodrigo Fernández-Quevedo García, Enrique Chacón, Pedro Tarazona and Chantal Valeriani","doi":"10.1039/D5SM00134J","DOIUrl":null,"url":null,"abstract":"<p >Adding a small amount of passive (Brownian) particles to a two-dimensional dense suspension of repulsive active Brownian particles does not affect the appearance of a motility-induced phase separation into a dense and a dilute phase, caused by the persistence of the active particles' direction of motion. Unlike a purely active suspension, the dense slab formed in an elongated system of a passive–active mixture may show, over long periods of time, a stable and well-defined propagation of the interfaces, because of the symmetry breaking caused by the depletion of passive particles on one side of the slab. We investigate these dynamical structures <em>via</em> average density profile calculations, revealing an asymmetry between the two interfaces, and enabling a kinetic analysis of the slab movement. The apparent movement of the dense slab is not a pure source/sink effect, nor a rigid displacement of all the particles, but a self-sustained combination of both effects. Furthermore, we analyse the specific fluctuations that produce, cancel and abruptly reverse the slab motion.</p>","PeriodicalId":103,"journal":{"name":"Soft Matter","volume":" 27","pages":" 5413-5422"},"PeriodicalIF":2.8000,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2025/sm/d5sm00134j?page=search","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Soft Matter","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/sm/d5sm00134j","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

Abstract

Adding a small amount of passive (Brownian) particles to a two-dimensional dense suspension of repulsive active Brownian particles does not affect the appearance of a motility-induced phase separation into a dense and a dilute phase, caused by the persistence of the active particles' direction of motion. Unlike a purely active suspension, the dense slab formed in an elongated system of a passive–active mixture may show, over long periods of time, a stable and well-defined propagation of the interfaces, because of the symmetry breaking caused by the depletion of passive particles on one side of the slab. We investigate these dynamical structures via average density profile calculations, revealing an asymmetry between the two interfaces, and enabling a kinetic analysis of the slab movement. The apparent movement of the dense slab is not a pure source/sink effect, nor a rigid displacement of all the particles, but a self-sustained combination of both effects. Furthermore, we analyse the specific fluctuations that produce, cancel and abruptly reverse the slab motion.

Abstract Image

掺杂运动诱导相分离的动力学和断裂。
将少量的被动(布朗)粒子加入到排斥性活性布朗粒子的二维密集悬浮液中,并不影响由活性粒子运动方向的持久性引起的运动诱导相分离为致密相和稀相的外观。与纯粹的主动悬架不同,在被动-主动混合物的细长系统中形成的致密板可能在很长一段时间内显示出界面的稳定和明确的传播,这是由于板的一侧被动粒子耗尽引起的对称性破坏。我们通过平均密度剖面计算来研究这些动力结构,揭示了两个界面之间的不对称性,并使板坯运动的动力学分析成为可能。致密板的表观运动不是纯粹的源/汇效应,也不是所有粒子的刚性位移,而是两种效应的自我持续组合。此外,我们还分析了产生、抵消和突然逆转平板运动的具体波动。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信