Deep transfer learning enabled online state-of-health estimation of lithium-ion batteries under small samples across different cathode materials, ambient temperature and charge-discharge protocols

IF 7.9 2区 工程技术 Q1 CHEMISTRY, PHYSICAL
Xiaopeng Li , Minghang Zhao , Shisheng Zhong , Junfu Li , Zhiquan Cui , Song Fu , Zhiqi Yan
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引用次数: 0

Abstract

State-of-health (SOH) estimation of lithium-ion batteries is crucial for ensuring their efficient and safe operation. However, the accurate SOH estimation under low temperatures and high discharge rates is still a challenging problem especially when facing insufficient early-stage data. To tackle this problem, this paper proposes a self-attention-based deep transfer learning (SDTL) approach that can be flexibly updated in respond to diverse cathode materials and varied operation conditions. First, an efficient self-attention-based feature learning model is constructed to capture diverse degradation patterns of batteries under different operating conditions. Second, deep transfer learning techniques are employed to achieve adaptable SOH estimation using previously learned degradation knowledge and the limited data of a new battery. To comprehensively validate the proposed approach, full life cycle tests on nickel cobalt manganese (NCM) batteries under 1C/2C conditions are conducted to supplement the nickel cobalt aluminum (NCA) public battery datasets. All the prepared battery datasets cover different cathode materials, charge-discharge rates, and ambient temperatures. Afterwards, eighteen health indicators are extracted and selected with Pearson correlation coefficient (PCC) to comprehensively characterize the statistical, electrochemical, and dynamic properties of batteries. Through comparisons with classical models that directly trained using state-of-the-art deep learning algorithms and other widely used deep transfer learning methods, the proposed SOH estimation approach has shown wide generalizability as well as a positive accuracy improvement.
深度迁移学习可以在不同正极材料、环境温度和充放电协议的小样本下在线估计锂离子电池的健康状态
锂离子电池的健康状态(SOH)评估是保证锂离子电池高效、安全运行的关键。然而,在低温和高排放速率下准确估算SOH仍然是一个具有挑战性的问题,特别是在早期数据不足的情况下。为了解决这一问题,本文提出了一种基于自注意的深度迁移学习(SDTL)方法,该方法可以灵活地更新以响应不同的阴极材料和不同的操作条件。首先,构建高效的基于自注意的特征学习模型,捕捉电池在不同工况下的各种退化模式;其次,利用之前学习到的退化知识和新电池的有限数据,采用深度迁移学习技术实现自适应SOH估计。为了全面验证所提出的方法,在1C/2C条件下对镍钴锰(NCM)电池进行了全生命周期测试,以补充镍钴铝(NCA)公共电池数据集。所有准备的电池数据集涵盖了不同的阴极材料、充放电速率和环境温度。然后,提取18个健康指标,并采用Pearson相关系数(PCC)对电池的统计、电化学和动态特性进行综合表征。通过与使用最先进的深度学习算法和其他广泛使用的深度迁移学习方法直接训练的经典模型的比较,所提出的SOH估计方法具有广泛的泛化性和积极的精度提高。
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来源期刊
Journal of Power Sources
Journal of Power Sources 工程技术-电化学
CiteScore
16.40
自引率
6.50%
发文量
1249
审稿时长
36 days
期刊介绍: The Journal of Power Sources is a publication catering to researchers and technologists interested in various aspects of the science, technology, and applications of electrochemical power sources. It covers original research and reviews on primary and secondary batteries, fuel cells, supercapacitors, and photo-electrochemical cells. Topics considered include the research, development and applications of nanomaterials and novel componentry for these devices. Examples of applications of these electrochemical power sources include: • Portable electronics • Electric and Hybrid Electric Vehicles • Uninterruptible Power Supply (UPS) systems • Storage of renewable energy • Satellites and deep space probes • Boats and ships, drones and aircrafts • Wearable energy storage systems
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