Dichotomous Temperature Response in the Electronic Structure of Epitaxially Grown Altermagnet MnTe

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Ji-Eun Lee*, Yong Zhong, Qile Li, Mark T. Edmonds, Zhi-Xun Shen, Choongyu Hwang and Sung-Kwan Mo*, 
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Abstract

The altermagnet candidate MnTe has recently gained significant interest due to its unconventional magnetic ordering. One of the key features of altermagnetism is the momentum-dependent spin-split band and its temperature-dependent evolution. Yet a fully momentum-resolved experimental investigation, including out-of-plane direction, is still lacking. Here, we systematically investigate the electronic structure of epitaxially grown MnTe by using angle-resolved photoemission spectroscopy (ARPES). Our photon-energy-dependent ARPES data reveal significant out-of-plane dispersions consistent with previous theoretical calculations. More interestingly, we identify two distinct temperature-dependent electronic band structure evolutions at different out-of-plane momentum positions: momentum-dependent energy shifts at the nodal plane and substantial spectral weight suppression at the off-nodal plane. These findings may suggest the importance of considering both the itinerant and localized nature of the magnetic ordering and momentum-dependent interactions. Our work provides crucial insights into the complex correlation between momentum, temperature, and electronic structure in MnTe, contributing to a deeper understanding of altermagnetism.

外延生长交变磁体MnTe电子结构的二元温度响应
交替磁体候选材料MnTe最近因其非常规的磁性排列而引起了极大的兴趣。变磁场的关键特征之一是动量依赖的自旋分裂带及其温度依赖的演化。然而,一个完全动量解决的实验研究,包括面外方向,仍然缺乏。本文采用角分辨光发射光谱(ARPES)系统地研究了外延生长MnTe的电子结构。我们的光子能量依赖的ARPES数据显示显著的面外色散与先前的理论计算一致。更有趣的是,我们在不同的面外动量位置发现了两种不同的温度相关电子能带结构演变:节点面上的动量相关能量转移和离节点面上的大量谱权抑制。这些发现可能表明考虑磁有序和动量依赖相互作用的流动和局部性质的重要性。我们的工作为MnTe中动量、温度和电子结构之间的复杂关系提供了重要的见解,有助于更深入地理解电磁学。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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