Investigation on strengthening effect of metal foams in enlarged microchannels for heterogeneous liquid-liquid mass transfer

IF 3.9 3区 工程技术 Q3 ENERGY & FUELS
Zhaoyang Shen , Qichao Wang , Feng Xu , Xiang Zhou , Lei Ni , Zhiquan Cheng , Juncheng Jiang
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Abstract

In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s-1. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.

Abstract Image

扩大微通道中金属泡沫强化液-液非均质传质效果的研究
在本研究中,为了增强放大微通道中两个非均相之间的传质过程,将金属泡沫填充到石英通道中。首先,采用均相碘酸盐体系研究了金属泡沫中流体的混合效率。结果表明,随着金属泡沫长度和孔隙密度的增加,混合效率提高。其次,采用正丁醇-丁二酸(非均相)体系研究了金属泡沫的萃取和传质效率。结果表明,孔径密度为60 PPI、长度为10 cm的金属泡沫的萃取效率和传质性能最好,分别达到56%和0.297 s-1;最后,采用硫化苯氧化工艺考察了金属泡沫对反应过程的增强作用,选择了传质性能最好的金属泡沫进行实验。在停留时间为15 min时,原料转化率达到86.57%,比无结构嵌套的通道提高了近4倍。因此,利用金属泡沫填充的放大微通道来加强传质过程是一种非常有意义的策略。
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来源期刊
CiteScore
7.80
自引率
9.30%
发文量
408
审稿时长
49 days
期刊介绍: Chemical Engineering and Processing: Process Intensification is intended for practicing researchers in industry and academia, working in the field of Process Engineering and related to the subject of Process Intensification.Articles published in the Journal demonstrate how novel discoveries, developments and theories in the field of Process Engineering and in particular Process Intensification may be used for analysis and design of innovative equipment and processing methods with substantially improved sustainability, efficiency and environmental performance.
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