Ultrasharp, Cavity Enhanced, Broadly Tunable Infrared Detection Using Colloidal Quantum Dots

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Erwan Bossavit, Dario Mastrippolito, Clement Gureghian, Albin Colle, Dries De Pesseroey, Marco Paye, Kseniia Sergeeva, Mariarosa Cavallo, Yanjun Ma, Adrien Khalili, Tommaso Gemo, Yoann Prado, Mohamad Hamieh, Erwan Dandeu, Sandrine Ithurria, Debora Pierucci, Mathieu G. Silly, Xavier Lafosse, Emmanuel Lhuillier
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Abstract

After the success of semiconductor nanocrystals as light sources for displays in the visible range, the infrared range now offers a complementary playground. Applications requiring chemical contrast in images and applications to LIDAR technology incentivize the development of devices with narrow spectral responses. However, the solutions that rely on introducing notch filters still suffer from imperfect transmission at the wavelength of interest in a spectral range where their detection is already difficult. Here, we explore the integration of a short-wave infrared detector directly into a dielectric microcavity. Our approach simultaneously achieves ultranarrow absorption lines below 30 cm–1 at a telecom wavelength, together with a broadband, continuous, postfabrication spectral tunability over 1200 cm–1. By taking advantage of the field magnification inside the cavity, we demonstrate that the spectral shaping properties can be obtained while maintaining performances on par with an uncoupled device, stressing the benefit of this method compared to filter-only approaches.

Abstract Image

使用胶体量子点的超尖锐、腔增强、宽可调谐红外探测
在半导体纳米晶体作为可见范围内显示器的光源成功之后,红外范围现在提供了一个互补的游乐场。需要图像化学对比的应用和激光雷达技术的应用激励了窄光谱响应设备的发展。然而,依赖于引入陷波滤波器的解决方案仍然会在感兴趣的波长上遭受不完美的传输,在光谱范围内,它们的检测已经很困难。在这里,我们探索将短波红外探测器直接集成到介电微腔中。我们的方法同时实现了电信波长30 cm-1以下的超窄吸收线,以及1200 cm-1以上的宽带、连续、后期光谱可调性。通过利用腔内的场放大,我们证明了在保持与非耦合器件相当的性能的同时可以获得光谱整形特性,强调了与仅使用滤波器的方法相比,这种方法的优点。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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