{"title":"Ultrasharp, Cavity Enhanced, Broadly Tunable Infrared Detection Using Colloidal Quantum Dots","authors":"Erwan Bossavit, Dario Mastrippolito, Clement Gureghian, Albin Colle, Dries De Pesseroey, Marco Paye, Kseniia Sergeeva, Mariarosa Cavallo, Yanjun Ma, Adrien Khalili, Tommaso Gemo, Yoann Prado, Mohamad Hamieh, Erwan Dandeu, Sandrine Ithurria, Debora Pierucci, Mathieu G. Silly, Xavier Lafosse, Emmanuel Lhuillier","doi":"10.1021/acs.nanolett.5c02212","DOIUrl":null,"url":null,"abstract":"After the success of semiconductor nanocrystals as light sources for displays in the visible range, the infrared range now offers a complementary playground. Applications requiring chemical contrast in images and applications to LIDAR technology incentivize the development of devices with narrow spectral responses. However, the solutions that rely on introducing notch filters still suffer from imperfect transmission at the wavelength of interest in a spectral range where their detection is already difficult. Here, we explore the integration of a short-wave infrared detector directly into a dielectric microcavity. Our approach simultaneously achieves ultranarrow absorption lines below 30 cm<sup>–1</sup> at a telecom wavelength, together with a broadband, continuous, postfabrication spectral tunability over 1200 cm<sup>–1</sup>. By taking advantage of the field magnification inside the cavity, we demonstrate that the spectral shaping properties can be obtained while maintaining performances on par with an uncoupled device, stressing the benefit of this method compared to filter-only approaches.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"19 1","pages":""},"PeriodicalIF":9.1000,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.5c02212","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
After the success of semiconductor nanocrystals as light sources for displays in the visible range, the infrared range now offers a complementary playground. Applications requiring chemical contrast in images and applications to LIDAR technology incentivize the development of devices with narrow spectral responses. However, the solutions that rely on introducing notch filters still suffer from imperfect transmission at the wavelength of interest in a spectral range where their detection is already difficult. Here, we explore the integration of a short-wave infrared detector directly into a dielectric microcavity. Our approach simultaneously achieves ultranarrow absorption lines below 30 cm–1 at a telecom wavelength, together with a broadband, continuous, postfabrication spectral tunability over 1200 cm–1. By taking advantage of the field magnification inside the cavity, we demonstrate that the spectral shaping properties can be obtained while maintaining performances on par with an uncoupled device, stressing the benefit of this method compared to filter-only approaches.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.