The Development and Evaluation of Hybrid Solar Cells Based on Perovskites and CIGS with Different ETL for Increased Photovoltaic Efficiency Using SCAPS-1D

IF 3.9 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Md. Abdul Monnaf, Avijit Ghosh*, Saeed Hasan Nabil, Md Baharul Islam, Tamanna Rashid, Abdullah Al Fathah, Khorshed Alam, Huriyyah A. Alturaifi and Nasser S. Awwad, 
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引用次数: 0

Abstract

The SCAPS-1D method has been utilized to simulate a solar panel with two absorber layers computationally. Implementing the hole transporter in the current work is minimized by employing two absorber layers. Structure of lead-based perovskites Simulations are conducted using copper indium gallium selenide (CIGS) and strontium arsenide iodide (Sr3AsI3). By combining perovskites’ high absorption coefficient and tunable bandgap with the stability and improved charge transport capabilities of CIGS, these bilayer solar cells can overcome the limitations of each material. Several factors are considered to attain maximum and enhanced efficiency, including absorber thickness, series-shunt resistance, acceptor density, defect densities, JV & QE, and operating temperature. The structure of the optimized device Al/Sr3AsI3/CIGS/SnS2/Ni produces excellent output with an efficiency of 35.91%, a voltage in the open circuit (VOC) of 0.998 V, a fill factor (FF) of 86.60%, and current in a short circuit (JSC) of 41.54 mA/cm2. This study demonstrates the promise of perovskite/CIGS double-layers as a means of achieving stable, scalable, and highly efficient thin-film photovoltaics. Comparing the results with previously published experimental data showed that the device might achieve excellent performance by fine-tuning various absorber layer settings. Therefore, this gadget structure is amenable to experimental modeling for future investigation. The simulation’s findings offer helpful suggestions for developing double-absorber solar panels. This paper examines the latest developments in perovskite/CIGS bilayers, addressing issues with scalability, long-term stability, and material compatibility. The findings show that, with further modification, perovskite/CIGS bilayer cells offer a lot of potential for next-generation solar power applications.

Abstract Image

基于不同ETL的钙钛矿和CIGS混合太阳能电池的开发与评价,以提高SCAPS-1D的光伏效率
利用SCAPS-1D方法对具有两层吸收层的太阳能电池板进行了数值模拟。通过采用两层吸收层,可以最大限度地减少当前工作中空穴传输体的使用。采用硒化铜铟镓(CIGS)和碘化砷化锶(Sr3AsI3)对铅基钙钛矿的结构进行了模拟。通过将钙钛矿的高吸收系数和可调带隙与CIGS的稳定性和改进的电荷传输能力相结合,这些双层太阳能电池可以克服每种材料的局限性。考虑了几个因素来获得最大和提高效率,包括吸收器厚度,串联分流电阻,受体密度,缺陷密度,J-V &;Q-E和工作温度。优化后的Al/Sr3AsI3/CIGS/SnS2/Ni器件的输出效率为35.91%,开路电压(VOC)为0.998 V,填充系数(FF)为86.60%,短路电流(JSC)为41.54 mA/cm2。这项研究表明,钙钛矿/CIGS双层材料有望成为实现稳定、可扩展和高效薄膜光伏发电的一种手段。结果与先前发表的实验数据比较表明,该装置可以通过微调各种吸收层设置来获得优异的性能。因此,该小工具结构适合于实验建模,以供将来的研究。模拟结果为开发双吸收板提供了有益的建议。本文研究了钙钛矿/CIGS双层膜的最新发展,解决了可扩展性,长期稳定性和材料兼容性问题。研究结果表明,通过进一步的修饰,钙钛矿/CIGS双层电池为下一代太阳能发电应用提供了很大的潜力。
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来源期刊
Langmuir
Langmuir 化学-材料科学:综合
CiteScore
6.50
自引率
10.30%
发文量
1464
审稿时长
2.1 months
期刊介绍: Langmuir is an interdisciplinary journal publishing articles in the following subject categories: Colloids: surfactants and self-assembly, dispersions, emulsions, foams Interfaces: adsorption, reactions, films, forces Biological Interfaces: biocolloids, biomolecular and biomimetic materials Materials: nano- and mesostructured materials, polymers, gels, liquid crystals Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do? Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*. This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).
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