Refractive Index Sensitive Coupling of Monolayer MoS2 and Plasmonic Heterostructure: Effect of Unit Cell Geometry

Anindita Mondal, Agnimitra Sutradhar and Abha Misra*, 
{"title":"Refractive Index Sensitive Coupling of Monolayer MoS2 and Plasmonic Heterostructure: Effect of Unit Cell Geometry","authors":"Anindita Mondal,&nbsp;Agnimitra Sutradhar and Abha Misra*,&nbsp;","doi":"10.1021/acsaom.5c0007110.1021/acsaom.5c00071","DOIUrl":null,"url":null,"abstract":"<p >The optical response of monolayer molybdenum disulfide (MoS<sub>2</sub>) is recorded after coupling it with the plasmonic array of gold nanostructures of different unit cell geometry. The normalized reflection spectra are recorded in different refractive index media varying from 1.00 to 1.47. A unique dependence on the unit cell geometry of the plasmonic array is observed, where the dimer and dumbbell structures showed a sensitivity of 23.49 and 60.70 nm/RIU, respectively. The shift in A excitonic peak position in the reflectance spectra of plasmonic MoS<sub>2</sub> is more pronounced compared to the shift in the B excitonic peak. An improved absorption by A and B excitons was observed compared with monolayer MoS<sub>2</sub>. The concept of tailoring excitonic intensity paves a way towards opto-chemical sensing, as well as provides a platform for two-dimensional (2D) nano-optoelectronics applications.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 5","pages":"1097–1105 1097–1105"},"PeriodicalIF":0.0000,"publicationDate":"2025-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Optical Materials","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaom.5c00071","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

Abstract

The optical response of monolayer molybdenum disulfide (MoS2) is recorded after coupling it with the plasmonic array of gold nanostructures of different unit cell geometry. The normalized reflection spectra are recorded in different refractive index media varying from 1.00 to 1.47. A unique dependence on the unit cell geometry of the plasmonic array is observed, where the dimer and dumbbell structures showed a sensitivity of 23.49 and 60.70 nm/RIU, respectively. The shift in A excitonic peak position in the reflectance spectra of plasmonic MoS2 is more pronounced compared to the shift in the B excitonic peak. An improved absorption by A and B excitons was observed compared with monolayer MoS2. The concept of tailoring excitonic intensity paves a way towards opto-chemical sensing, as well as provides a platform for two-dimensional (2D) nano-optoelectronics applications.

单元化二硫化钼与等离子异质结构的折射率敏感耦合:单元胞几何的影响
将单层二硫化钼(MoS2)与不同单元几何形状的金纳米结构等离子体阵列耦合后,记录了其光学响应。在折射率为1.00 ~ 1.47的介质中记录了归一化反射光谱。等离子体阵列具有独特的几何特性,其中二聚体和哑铃结构的灵敏度分别为23.49和60.70 nm/RIU。等离子体MoS2反射光谱中A激子峰位置的移位比B激子峰位置的移位更为明显。与单层MoS2相比,观察到A和B激子的吸收有所改善。定制激子强度的概念为光化学传感铺平了道路,并为二维(2D)纳米光电子应用提供了一个平台。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
ACS Applied Optical Materials
ACS Applied Optical Materials 材料科学-光学材料-
CiteScore
1.10
自引率
0.00%
发文量
0
期刊介绍: ACS Applied Optical Materials is an international and interdisciplinary forum to publish original experimental and theoretical including simulation and modeling research in optical materials complementing the ACS Applied Materials portfolio. With a focus on innovative applications ACS Applied Optical Materials also complements and expands the scope of existing ACS publications that focus on fundamental aspects of the interaction between light and matter in materials science including ACS Photonics Macromolecules Journal of Physical Chemistry C ACS Nano and Nano Letters.The scope of ACS Applied Optical Materials includes high quality research of an applied nature that integrates knowledge in materials science chemistry physics optical science and engineering.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信